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Solvothermal Synthesis and Photoreactivity of Anatase TiO2 Nanosheets with Dominant {001} Facets
Abstract
Owing to wide-ranging industrial applications and fundamental importance, tailored synthesis of well-faceted single crystals of anatase TiO(2) with high percentage of reactive facets has attracted much research interest. In this work, high-quality anatase TiO(2) single-crystal nanosheets mainly dominated by {001} facets have been prepared by using a water-2-propanol solvothermal synthetic route. The synergistic functions of 2-propanol and HF on the growth of anatase TiO(2) single-crystal nanosheets were studied by first-principle theoretical calculations, revealing that the addition of 2-propanol can strengthen the stabilization effect associated with fluorine adsorption over (001) surface and thus stimulate its preferred growth. By measuring the (*)OH species with terephthalic acid scavenger, the as-prepared anatase TiO(2) single-crystal nanosheets having 64% {001} facets show superior photoreactivity (more than 5 times), compared to P25 as a benchmarking material.
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Semiconductor-based Photocatalytic Hydrogen Generation
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TiO2 photocatalysis: Design and applications
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Why is anatase a better photocatalyst than rutile? - Model studies on epitaxial TiO2 films
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Self-citation
Metadata
- Authors
- Yang, H. G., Liu, G., Qiao, S. Z., Sun, C. H., Jin, Y. G., Smith, S. C., Zou, J., Cheng, H. M., & Lu, G. Q. (.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-02-27
- Volume
- 131
- Issue
- 11
- Pages
- 4078-4083
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1966719571
- Cited by
- 1,305
- References
- 6
- FWCI
- 47.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, H. G., Liu, G., Qiao, S. Z., Sun, C. H., Jin, Y. G., Smith, S. C., Zou, J., Cheng, H. M., & Lu, G. Q. (. (2009). Solvothermal Synthesis and Photoreactivity of Anatase TiO2 Nanosheets with Dominant {001} Facets. Journal of the American Chemical Society. https://doi.org/10.1021/ja808790p
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