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Temperature and Concentration Control over Interpenetration in a Metal−Organic Material
Abstract
A pillared framework formed from 4,4'-bipyridine (bipy) and sheets of dinuclear Cd(2) nodes and 1,4-benzenedicarboxylic acid (bdc) linkers can be prepared in both interpenetrated and noninterpenetrated forms by simply varying the temperature or concentration of the reaction. These results demonstrate that higher temperatures and concentrations favor interpenetration over the corresponding noninterpenetrating structure, an observation that could have broad implications for controlling the synthesis of metal-organic materials.
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Cited by
From fundamentals to applications: a toolbox for robust and multifunctional MOF materials
Kirchon, A., Feng, L., Drake, H. F., Joseph, E. A., & Zhou, H.-C. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00688a · Cited by 1,448
Yang, S., Lin, X., Lewis, W., Suyetin, M., Bichoutskaia, E., Parker, J. E., Tang, C. C., Allan, D. R., Rizkallah, P. J., Hubberstey, P., et al. (2012) · Nature Materials · doi:10.1038/nmat3343 · Cited by 477
Activation of metal–organic framework materials
Mondloch, J. E., Karagiaridi, O., Farha, O. K., & Hupp, J. T. (2013) · CrystEngComm · doi:10.1039/c3ce41232f · Cited by 324
In silico Design of Porous Polymer Networks: High-Throughput Screening for Methane Storage Materials
Martin, R. L., Simon, C. M., Smit, B., & Haranczyk, M. (2014) · Journal of the American Chemical Society · doi:10.1021/ja4123939 · Cited by 170
Metadata
- Authors
- Zhang, J., Wojtas, L., Larsen, R. W., Eddaoudi, M., & Zaworotko, M. J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-11-05
- Volume
- 131
- Issue
- 47
- Pages
- 17040-17041
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1981279976
- Cited by
- 388
- References
- 0
- FWCI
- 22.57
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, J., Wojtas, L., Larsen, R. W., Eddaoudi, M., & Zaworotko, M. J. (2009). Temperature and Concentration Control over Interpenetration in a Metal−Organic Material. Journal of the American Chemical Society. https://doi.org/10.1021/ja906911q
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