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Monodisperse Nickel Nanoparticles and Their Catalysis in Hydrolytic Dehydrogenation of Ammonia Borane
Open accessAbstract
Monodisperse nickel nanoparticles are prepared from the reduction of Ni(acac)(2) with borane tributylamine in the presence of oleylamine and oleic acid. Without any special treatment to remove the surfactants, the as-synthesized Ni nanoparticles supported on the Ketjen carbon support exhibit high catalytic activity in hydrogen generation from the hydrolysis of the ammonia-borane (H(3)NBH(3)) complex with a total turnover frequency value of 8.8 mol of H(2) x (mol of Ni)(-1) x min(-1). Such catalysis based on Ni nanoparticles represents a promising step toward the practical development of the H(3)NBH(3) complex as a feasible hydrogen storage medium for fuel cell applications.
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Cites
Materials for hydrogen storage
Züttel, A. (2003) · Materials Today · doi:10.1016/s1369-7021(03)00922-2 · Cited by 2,216
Ni1-xPtx (x = 0−0.12) Hollow Spheres as Catalysts for Hydrogen Generation from Ammonia Borane
Cheng, F., Ma, H., Li, Y., & Chen, J. (2007) · Inorganic Chemistry · doi:10.1021/ic061712e · Cited by 349
Cited by
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Wang, D., & Astruc, D. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00629a · Cited by 608
Organic Phase Syntheses of Magnetic Nanoparticles and Their Applications
Wu, L., Mendoza-Garcia, A., Li, Q., & Sun, S. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00687 · Cited by 601
Self-citationHou, C.-C., Li, Q., Wang, C.-J., Peng, C.-Y., Chen, Q.-Q., Ye, H.-F., Fu, W.-F., Che, C.-M., López, N., & Chen, Y. (2017) · Energy & Environmental Science · doi:10.1039/c7ee01553d · Cited by 267
Importance of Size and Distribution of Ni Nanoparticles for the Hydrodeoxygenation of Microalgae Oil
Song, W., Zhao, C., & Lercher, J. A. (2013) · Chemistry – A European Journal · doi:10.1002/chem.201301005 · Cited by 154
Specific Solvent Produces Specific Phase Ni Nanoparticles: A Pulsed Laser Ablation in Solvents
Jung, H. J., & Choi, M. Y. (2014) · The Journal of Physical Chemistry C · doi:10.1021/jp503009a · Cited by 93
Metadata
- Authors
- Metin, Ö., Mazumder, V., Özkar, S., & Sun, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-01-15
- Volume
- 132
- Issue
- 5
- Pages
- 1468-1469
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1991262398
- Cited by
- 515
- References
- 2
- FWCI
- 18.22
- Type
- journal article
- Language
- en
- Open access
- green
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- Metin, Ö., Mazumder, V., Özkar, S., & Sun, S. (2010). Monodisperse Nickel Nanoparticles and Their Catalysis in Hydrolytic Dehydrogenation of Ammonia Borane. Journal of the American Chemical Society. https://doi.org/10.1021/ja909243z
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