The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Photoinduced Strong Metal–Support Interaction for Enhanced Catalysis
Open accessAbstract
Strong metal–support interaction (SMSI) construction is a pivotal strategy to afford thermally robust nanocatalysts in industrial catalysis, but thermally induced reactions (>300 °C) in specific gaseous atmospheres are generally required in traditional procedures. In this work, a photochemistry-driven methodology was demonstrated for SMSI construction under ambient conditions. Encapsulation of Pd nanoparticles with a TiO x overlayer, the presence of Ti 3+ species, and suppression of CO adsorption were achieved upon UV irradiation. The key lies in the generation of separated photoinduced reductive electrons (e – ) and oxidative holes (h + ), which subsequently trigger the formation of Ti 3+ species/oxygen vacancies (O v ) and then interfacial Pd–O v –Ti 3+ sites, affording a Pd/TiO 2 SMSI with enhanced catalytic hydrogenation efficiency. The as-constructed SMSI layer was reversible, and the photodriven procedure could be extended to Pd/ZnO and Pt/TiO 2 .
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Cites
Strong metal-support interactions. Group 8 noble metals supported on titanium dioxide
Tauster, S. J., Fung, S. C., & Garten, R. L. (1978) · Journal of the American Chemical Society · doi:10.1021/ja00469a029 · Cited by 3,188
Surface Science Studies of the Photoactivation of TiO 2 New Photochemical Processes
Thompson, T. L., & Yates, J. T. (2006) · Chemical Reviews · doi:10.1021/cr050172k · Cited by 2,064
Cited by
Li, Y., Zhang, Y., Qian, K., & Huang, W. (2022) · ACS Catalysis · doi:10.1021/acscatal.1c04854 · Cited by 538
Metal–support interactions in metal oxide-supported atomic, cluster, and nanoparticle catalysis
Leybo, D., Etim, U. J., Monai, M., Bare, S. R., Zhong, Z., & Vogt, C. (2024) · Chemical Society Reviews · doi:10.1039/d4cs00527a · Cited by 417
Metadata
- Authors
- Chen, H., Yang, Z., Wang, X., Polo-Garzon, F., Halstenberg, P. W., Wang, T., Suo, X., Yang, S.-Z., Meyer, H. M., Wu, Z., & Dai, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-06-03
- Volume
- 143
- Issue
- 23
- Pages
- 8521-8526
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W3165548732
- Cited by
- 182
- References
- 2
- FWCI
- 11.19
- Type
- journal article
- Language
- en
- Open access
- green
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- Chen, H., Yang, Z., Wang, X., Polo-Garzon, F., Halstenberg, P. W., Wang, T., Suo, X., Yang, S.-Z., Meyer, H. M., Wu, Z., & Dai, S. (2021). Photoinduced Strong Metal–Support Interaction for Enhanced Catalysis. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.0c12817
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