The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Doping Shortens the Metal/Metal Distance and Promotes OH Coverage in Non-Noble Acidic Oxygen Evolution Reaction Catalysts
Open accessAbstract
Acidic water electrolysis enables the production of hydrogen for use as a chemical and as a fuel. The acidic environment hinders water electrolysis on non-noble catalysts, a result of the sluggish kinetics associated with the adsorbate evolution mechanism, reliant as it is on four concerted proton-electron transfer steps. Enabling a faster mechanism with non-noble catalysts will help to further advance acidic water electrolysis. Here, we report evidence that doping Ba cations into a Co 3 O 4 framework to form Co 3– x Ba x O 4 promotes the oxide path mechanism and simultaneously improves activity in acidic electrolytes. Co 3– x Ba x O 4 catalysts reported herein exhibit an overpotential of 278 mV at 10 mA/cm 2 in 0.5 M H 2 SO 4 electrolyte and are stable over 110 h of continuous water oxidation operation. We find that the incorporation of Ba cations shortens the Co–Co distance and promotes OH adsorption, findings we link to improved water oxidation in acidic electrolyte.
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Cites
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Self-citationReier, T., Nong, H. N., Teschner, D., Schlögl, R., & Strasser, P. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201601275 · Cited by 1,253
Han, N., Yang, K. R., Lu, Z., Li, Y., Xu, W., Gao, T., Cai, Z., Zhang, Y., Batista, V. S., Liu, W., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-03429-z · Cited by 766
Cited by
Stability of electrocatalytic OER: from principle to application
Li, H., Lin, Y., Duan, J., Wen, Q., Liu, Y., & Zhai, T. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00010a · Cited by 540
Self-citationRong, C., Huang, X., Arandiyan, H., Shao, Z., Wang, Y., & Chen, Y. (2025) · Advanced Materials · doi:10.1002/adma.202416362 · Cited by 333
Song, H., Yong, X., Waterhouse, G. I. N., Yu, J., Wang, H., Cai, J., Tang, Z., Yang, B., Chang, J., & Lu, S. (2024) · ACS Catalysis · doi:10.1021/acscatal.3c06182 · Cited by 280
Ji, Q., Tang, B., Zhang, X., Wang, C., Tan, H., Zhao, J., Liu, R., Sun, M., Liu, H., Jiang, C., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-52471-7 · Cited by 183
Dong, Z., Li, B., & Zhu, Y. (2024) · Energy & Fuels · doi:10.1021/acs.energyfuels.4c00837 · Cited by 66
Metadata
- Authors
- Wang, N., Ou, P., Miao, R. K., Chang, Y., Wang, Z., Hung, S.-F., Abed, J., Ozden, A., Chen, H.-Y., Wu, H.-L., Huang, J. E., Zhou, D., Ni, W., Fan, L., Yan, Y., Peng, T., Sinton, D., Liu, Y., Liang, H., & Sargent, E. H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2023-04-03
- Volume
- 145
- Issue
- 14
- Pages
- 7829-7836
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W4362506256
- Cited by
- 314
- References
- 3
- FWCI
- 14.70
- Type
- journal article
- Language
- en
- Open access
- green
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- Wang, N., Ou, P., Miao, R. K., Chang, Y., Wang, Z., Hung, S.-F., Abed, J., Ozden, A., Chen, H.-Y., Wu, H.-L., Huang, J. E., Zhou, D., Ni, W., Fan, L., Yan, Y., Peng, T., Sinton, D., Liu, Y., Liang, H., & Sargent, E. H. (2023). Doping Shortens the Metal/Metal Distance and Promotes OH Coverage in Non-Noble Acidic Oxygen Evolution Reaction Catalysts. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.2c12431
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