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Charge Transfer Excitons at van der Waals Interfaces
Open accessAbstract
The van der Waals interfaces of molecular donor/acceptor or graphene-like two-dimensional (2D) semiconductors are central to concepts and emerging technologies of light-electricity interconversion. Examples include, among others, solar cells, photodetectors, and light emitting diodes. A salient feature in both types of van der Waals interfaces is the poorly screened Coulomb potential that can give rise to bound electron-hole pairs across the interface, i.e., charge transfer (CT) or interlayer excitons. Here we address common features of CT excitons at both types of interfaces. We emphasize the competition between localization and delocalization in ensuring efficient charge separation. At the molecular donor/acceptor interface, electronic delocalization in real space can dictate charge carrier separation. In contrast, at the 2D semiconductor heterojunction, delocalization in momentum space due to strong exciton binding may assist in parallel momentum conservation in CT exciton formation.
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Cites
Spin and pseudospins in layered transition metal dichalcogenides
Xu, X., Yao, W., Xiao, D., & Heinz, T. F. (2014) · Nature Physics · doi:10.1038/nphys2942 · Cited by 2,855
Entropy of Charge Separation in Organic Photovoltaic Cells: The Benefit of Higher Dimensionality
Gregg, B. A. (2011) · The Journal of Physical Chemistry Letters · doi:10.1021/jz2012403 · Cited by 245
Cited by
Acharya, R., & Parida, K. (2020) · Journal of Environmental Chemical Engineering · doi:10.1016/j.jece.2020.103896 · Cited by 462
Zheng, Q., Chu, W., Zhao, C., Zhang, L., Guo, H., Wang, Y., Jiang, X., & Zhao, J. (2019) · WIREs Computational Molecular Science · doi:10.1002/wcms.1411 · Cited by 452
Ultrafast formation of interlayer hot excitons in atomically thin MoS2/WS2 heterostructures
Chen, H., Wen, X., Zhang, J., Wu, T., Gong, Y., Zhang, X., Yuan, J., Yi, C., Lou, J., Ajayan, P. M., et al. (2016) · Nature Communications · doi:10.1038/ncomms12512 · Cited by 432
Metadata
- Authors
- Zhu, X., Monahan, N. R., Gong, Z., Zhu, H., Williams, K. W., & Nelson, C. A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-06-15
- Volume
- 137
- Issue
- 26
- Pages
- 8313-8320
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W341387266
- Cited by
- 305
- References
- 2
- FWCI
- 12.39
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Zhu, X., Monahan, N. R., Gong, Z., Zhu, H., Williams, K. W., & Nelson, C. A. (2015). Charge Transfer Excitons at van der Waals Interfaces. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b03141
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