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Entropy of Charge Separation in Organic Photovoltaic Cells: The Benefit of Higher Dimensionality
Abstract
The role of entropy in charge separation processes is discussed with respect to the dimensionality of the organic semiconductor. In 1-D materials, the change in entropy, Δ S, plays no role, but at higher dimensions, it leads to a substantial decrease in the Coulomb barrier for charge separation. The effects of Δ S are highest in equilibrium systems but decrease and become time-dependent in illuminated organic photovoltaic (OPV) cells. Higher-dimensional semiconductors have inherent advantages for charge separation, and this may be one reason that C 60 and its derivatives, the only truly three-dimensional organic semiconductors yet known, play such an important role in OPV cells.
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Some materials with 3D architectures showed better performance than their planar counterparts due to multi-directional charge-transport.
“It is generally accepted that some materials with 3D architectures showed better performance than their planar counterparts 122 due to the multi-directional charge-transport,”
From Recent progress in porphyrin-based materials for organic solar cells (2018) · cites this paper as [123]
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Metadata
- Authors
- Gregg, B. A.
- Affiliations
- National Laboratory of the Rockies (US)
- Corresponding author
- Gregg, Brian A.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-11-18
- Volume
- 2
- Issue
- 24
- Pages
- 3013-3015
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2323662954
- Cited by
- 245
- References
- 8
- Citations by year
- 2026: 2 · 2025: 4 · 2024: 11 · 2023: 12 · 2022: 10 · 2021: 18 · 2020: 20 · 2019: 21 · 2018: 31 · 2017: 23 · 2016: 28 · 2015: 28 · 2014: 18 · 2013: 12 · 2012: 6
- FWCI
- 8.29
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- The Journal of Physical Chemistry Letters (publishedVersion)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Electronics and Photovoltaics
- Physical Sciences › Chemistry › Organic Chemistry › Fullerene Chemistry and Applications
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Photochemistry and Electron Transfer Studies
- Keywords
- entropy, charge separation, organic solar cells, organic semiconductors, dimensionality, Coulomb barrier, C60, excited-state dynamics
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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