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RbMgCO3F: A New Beryllium-Free Deep-Ultraviolet Nonlinear Optical Material
Abstract
A new deep-ultraviolet nonlinear optical material, RbMgCO3F, has been synthesized and characterized. The achiral nonpolar acentric material is second harmonic generation (SHG) active at both 1064 and 532 nm, with efficiencies of 160 × α-SiO2 and 0.6 × β-BaB2O4, respectively, and exhibits a short UV cutoff, below 190 nm. RbMgCO3F possesses a three-dimensional structure of corner-shared Mg(CO3)2F2 polyhedra. Unlike other acentric carbonate fluorides, in this example, the inclusion of Mg(2+) creates pentagonal channels where the Rb(+) resides. Our electronic structure calculations reveal that the denticity of the carbonate linkage, monodentate or bidendate, to the divalent cation is a useful parameter for tuning the transparency window and achieving the sizable SHG response.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Cited by
Ok, K. M. (2016) · Accounts of Chemical Research · doi:10.1021/acs.accounts.6b00452 · Cited by 601
Two Non-π-Conjugated Deep-UV Nonlinear Optical Sulfates
Li, Y., Liang, F., Zhao, S., Li, L., Wu, Z., Ding, Q., Liu, S., Lin, Z., Hong, M., & Luo, J. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b00138 · Cited by 268
Metadata
- Authors
- Tran, T. T., He, J., Rondinelli, J. M., & Halasyamani, P. S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-08-14
- Volume
- 137
- Issue
- 33
- Pages
- 10504-10507
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2201805567
- Cited by
- 341
- References
- 1
- FWCI
- 12.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tran, T. T., He, J., Rondinelli, J. M., & Halasyamani, P. S. (2015). RbMgCO3F: A New Beryllium-Free Deep-Ultraviolet Nonlinear Optical Material. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b06519
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