The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Noncovalent Immobilization of a Molecular Iron-Based Electrocatalyst on Carbon Electrodes for Selective, Efficient CO2-to-CO Conversion in Water
Abstract
Catalysis of fuel-producing reactions can be transferred from homogeneous solution to surface via attachment of the molecular catalyst. A pyrene-appended iron triphenyl porphyrin bearing six pendant OH groups on the phenyl rings in all ortho and ortho' positions was immobilized on carbon nanotubes via noncovalent interactions and further deposited on glassy carbon. X-ray photoelectron spectroscopy and electrochemistry confirm catalyst immobilization. Using the carbon material, highly selective and rapid catalysis of the reduction of CO2 into CO occurs in water (pH 7.3) with 480 mV overpotential. Catalysis could be sustained for hours without loss of activity and selectivity, and high turnover number was obtained.
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Cites
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
The Fischer-Tropsch process: 1950-2000
Dry, M. E. (2002) · Catalysis Today · doi:10.1016/s0920-5861(01)00453-9 · Cited by 2,061
Cited by
Electro- and Solar-Driven Fuel Synthesis with First Row Transition Metal Complexes
Dalle, K. E., Warnan, J., Leung, J. J., Reuillard, B., Karmel, I. S., & Reisner, E. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00392 · Cited by 912
Wang, Y.-R., Huang, Q., He, C.-T., Chen, Y., Liu, J., Shen, F.-C., & Lan, Y.-Q. (2018) · Nature Communications · doi:10.1038/s41467-018-06938-z · Cited by 482
Electrocatalytic reduction of carbon dioxide: opportunities with heterogeneous molecular catalysts
Sun, L., Reddu, V., Fisher, A. C., & Wang, X. (2020) · Energy & Environmental Science · doi:10.1039/c9ee03660a · Cited by 452
Boutin, E., Merakeb, L., Ma, B., Boudy, B., Wang, M., Bonin, J., Anxolabéhère-Mallart, E., & Robert, M. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00218f · Cited by 423
Self-citationCovalently Grafting Cobalt Porphyrin onto Carbon Nanotubes for Efficient CO2 Electroreduction
Zhu, M., Chen, J., Huang, L., Ye, R., Xu, J., & Han, Y. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201900499 · Cited by 267
Metadata
- Authors
- Maurin, A., & Robert, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-22
- Volume
- 138
- Issue
- 8
- Pages
- 2492-2495
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2282560653
- Cited by
- 307
- References
- 2
- FWCI
- 10.37
- Type
- journal article
- Language
- en
- Open access
- closed
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- Maurin, A., & Robert, M. (2016). Noncovalent Immobilization of a Molecular Iron-Based Electrocatalyst on Carbon Electrodes for Selective, Efficient CO2-to-CO Conversion in Water. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b12652
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