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Synthesis of 4H/fcc Noble Multimetallic Nanoribbons for Electrocatalytic Hydrogen Evolution Reaction
Abstract
Noble multimetallic nanomaterials, if only consisting of Au, Ag, Pt, and Pd, typically adopt the high-symmetry face-centered cubic (fcc) structure. Here for the first time, by using the 4H/fcc Au@Ag nanoribbons (NRBs) as seeds, we report the synthesis of 4H/fcc trimetallic Au@PdAg core-shell NRBs via the galvanic reaction method under ambient conditions. Moreover, this strategy can also be used to synthesize 4H/fcc trimetallic Au@PtAg and quatermetallic Au@PtPdAg core-shell NRBs. Impressively, for the first time, these alloy shells, i.e., PdAg, PtAg, and PtPdAg, epitaxially grown on the 4H/fcc Au core with novel 4H hexagonal phase were successfully synthesized. Remarkably, the obtained 4H/fcc Au@PdAg NRBs exhibit excellent electrocatalytic activity toward the hydrogen evolution reaction, which is even quite close to that of the commercial Pt black. We believe that our findings here may provide a novel strategy for the crystal-structure-controlled synthesis of advanced functional noble multimetallic nanomaterials with various promising applications.
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Tian, N., Zhou, Z.-Y., Sun, S.-G., Ding, Y., & Wang, Z. L. (2007) · Science · doi:10.1126/science.1140484 · Cited by 3,073
Ghosh, T., Vukmirovic, M. B., DiSalvo, F. J., & Adzic, R. R. (2010) · Journal of the American Chemical Society · doi:10.1021/ja905850c · Cited by 141
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Self-citationShi, Y., Zhou, Y., Yang, D.-R., Xu, W.-X., Wang, C., Wang, F.-B., Xu, J.-J., Xia, X.-H., & Chen, H.-Y. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b08881 · Cited by 891
Wang, P., Zhang, X., Zhang, J., Wan, S., Guo, S., Lu, G., Yao, J., & Huang, X. (2017) · Nature Communications · doi:10.1038/ncomms14580 · Cited by 860
Self-citationEnhancing Electrocatalytic Water Splitting by Strain Engineering
You, B., Tang, M. T., Tsai, C., Abild‐Pedersen, F., Zheng, X., & Li, H. (2019) · Advanced Materials · doi:10.1002/adma.201807001 · Cited by 793
Long, R., Li, Y., Liu, Y., Chen, S., Zheng, X., Gao, C., He, C., Chen, N., Qi, Z., Song, L., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b00452 · Cited by 571
Metadata
- Authors
- Fan, Z., Luo, Z., Huang, X., Li, B., Chen, Y., Wang, J., Hu, Y., & Zhang, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-01-22
- Volume
- 138
- Issue
- 4
- Pages
- 1414-1419
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2237932705
- Cited by
- 214
- References
- 2
- FWCI
- 8.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fan, Z., Luo, Z., Huang, X., Li, B., Chen, Y., Wang, J., Hu, Y., & Zhang, H. (2016). Synthesis of 4H/fcc Noble Multimetallic Nanoribbons for Electrocatalytic Hydrogen Evolution Reaction. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b12715
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