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Design and Synthesis of New Circularly Polarized Thermally Activated Delayed Fluorescence Emitters
Open accessAbstract
This work describes the first thermally activated delayed fluorescence material enabling circularly polarized light emission through chiral perturbation. These new molecular architectures obtained through a scalable one-pot sequential synthetic procedure at room temperature (83% yield) display high quantum yield (up to 74%) and circularly polarized luminescence with an absolute luminescence dissymmetry factor, |glum|, of 1.3 × 10(-3). These chiral molecules have been used as an emissive dopant in an organic light emitting diode exhibiting external quantum efficiency as high as 9.1%.
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Cited by
Recent advances in organic thermally activated delayed fluorescence materials
Yang, Z., Mao, Z., Xie, Z., Zhang, Y., Liu, S., Zhao, J., Xu, J., Chi, Z., & Aldred, M. P. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00368k · Cited by 2,395
Circularly Polarized Luminescence in Nanoassemblies: Generation, Amplification, and Application
Sang, Y., Han, J., Zhao, T., Duan, P., & Liu, M. (2020) · Advanced Materials · doi:10.1002/adma.201900110 · Cited by 1,162
Design of Lanthanide‐Based OLEDs with Remarkable Circularly Polarized Electroluminescence
Zinna, F., Pasini, M., Galeotti, F., Botta, C., Di Bari, L., & Giovanella, U. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201603719 · Cited by 423
Yang, S.-Y., Wang, Y.-K., Peng, C.-C., Wu, Z.-G., Yuan, S., Yu, Y.-J., Li, H., Wang, T.-T., Li, H.-C., Zheng, Y.-X., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c08980 · Cited by 322
Metadata
- Authors
- Feuillastre, S., Pauton, M., Gao, L., Desmarchelier, A., Riives, A. J., Prim, D., Tondelier, D., Geffroy, B., Muller, G., Clavier, G., & Pieters, G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-18
- Volume
- 138
- Issue
- 12
- Pages
- 3990-3993
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2296508261
- Cited by
- 374
- References
- 0
- FWCI
- 15.09
- Type
- journal article
- Language
- en
- Open access
- green
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- Feuillastre, S., Pauton, M., Gao, L., Desmarchelier, A., Riives, A. J., Prim, D., Tondelier, D., Geffroy, B., Muller, G., Clavier, G., & Pieters, G. (2016). Design and Synthesis of New Circularly Polarized Thermally Activated Delayed Fluorescence Emitters. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b00850
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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