The DOI matches its Crossref record; 41 of the 41 references it cites were found in a registry or an index.
Constructing Solid–Gas-Interfacial Fenton Reaction over Alkalinized-C3N4 Photocatalyst To Achieve Apparent Quantum Yield of 49% at 420 nm
Abstract
Efficient generation of active oxygen-related radicals plays an essential role in boosting advanced oxidation process. To promote photocatalytic oxidation for gaseous pollutant over g-C 3 N 4, a solid–gas interfacial Fenton reaction is coupled into alkalinized g-C 3 N 4 -based photocatalyst to effectively convert photocatalytic generation of H 2 O 2 into oxygen-related radicals. This system includes light energy as power, alkalinized g-C 3 N 4 -based photocatalyst as an in situ and robust H 2 O 2 generator, and surface-decorated Fe 3+ as a trigger of H 2 O 2 conversion, which attains highly efficient and universal activity for photodegradation of volatile organic compounds (VOCs). Taking the photooxidation of isopropanol as model reaction, this system achieves a photoactivity of 2–3 orders of magnitude higher than that of pristine g-C 3 N 4, which corresponds to a high apparent quantum yield of 49% at around 420 nm. In-situ electron spin resonance (ESR) spectroscopy and sacrificial-reagent incorporated photocatalytic characterizations indicate that the notable photoactivity promotion could be ascribed to the collaboration between photocarriers (electrons and holes) and Fenton process to produce abundant and reactive oxygen-related radicals. The strategy of coupling solid–gas interfacial Fenton process into semiconductor-based photocatalysis provides a facile and promising solution to the remediation of air pollution via solar energy.
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Cited by
Yang, Y., Li, X., Zhou, C., Xiong, W., Zeng, G., Huang, D., Zhang, C., Wang, W., Song, B., Tang, X., et al. (2020) · Water Research · doi:10.1016/j.watres.2020.116200 · Cited by 518
Photocatalytic H2O2 production Systems: Design strategies and environmental applications
Chen, Z., Yao, D., Chu, C., & Mao, S. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.138489 · Cited by 482
Ong, W.-J., Putri, L. K., Tan, Y.-C., Tan, L.-L., Li, N., Ng, Y. H., Wen, X., & Chai, S.-P. (2017) · Nano Research · doi:10.1007/s12274-016-1391-4 · Cited by 470
Graphitic carbon nitrides (g-C3N4) with comparative discussion to carbon materials
Inagaki, M., Tsumura, T., Kinumoto, T., & Toyoda, M. (2019) · Carbon · doi:10.1016/j.carbon.2018.09.082 · Cited by 401
Zhang, D., Guo, Y., & Zhao, Z. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2017.12.044 · Cited by 357
Metadata
- Authors
- Li, Y., Ouyang, S., Xu, H., Wang, X., Bi, Y., Zhang, Y., & Ye, J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-10-03
- Volume
- 138
- Issue
- 40
- Pages
- 13289-13297
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2521750066
- Cited by
- 441
- References
- 41
- FWCI
- 14.93
- Type
- journal article
- Language
- en
- Open access
- closed
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