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A Micelle Fusion–Aggregation Assembly Approach to Mesoporous Carbon Materials with Rich Active Sites for Ultrasensitive Ammonia Sensing
Open accessAbstract
Nanostructured carbon materials have received considerable attention due to their special physicochemical properties. Herein, ordered mesoporous carbons (OMCs) with two-dimension (2D) hexagonal mesostructure and unique buckled large mesopores have successfully been synthesized via a micelle fusion-aggregation assembly method by using poly(ethylene oxide)-block-polystyrene (PEO-b-PS) diblock copolymers as a template and resorcinol-based phenolic resin as a carbon precursor. The obtained ordered mesoporous carbons possess unique fiber-like morphology, specific surface area of 571-880 m(2)/g, pore volume of 0.54 cm(3)/g and large mesopores (up to 36.3 nm) and high density of active sites (i.e., carboxylic groups) of 0.188/nm(2). Gas sensor based on the ordered mesoporous carbons exhibits an excellent performance in sensing NH3 at a low temperature with fast response (<2 min), ultralow limit of detection (<1 ppm), and good selectivity, due to the large pore sizes, high surface area and rich active sites in the carbon pore walls.
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Deng, Y., Yu, T., Wan, Y., Shi, Y., Meng, Y., Gu, D., Zhang, L., Huang, Y., Liu, C., Wu, X., et al. (2007) · Journal of the American Chemical Society · doi:10.1021/ja067379v · Cited by 402
Self-citationMesoscale assembly of chemically modified graphene into complex cellular networks
Barg, S., Perez, F. M., Ni, N., do Vale Pereira, P., Maher, R. C., Garcia-Tuñon, E., Eslava, S., Agnoli, S., Mattevi, C., & Saiz, E. (2014) · Nature Communications · doi:10.1038/ncomms5328 · Cited by 285
Cited by
Peng, L., Hung, C.-T., Wang, S., Zhang, X., Zhu, X., Zhao, Z., Wang, C., Tang, Y., Li, W., & Zhao, D. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b02091 · Cited by 607
Self-citationSurface and Interface Engineering of Silicon‐Based Anode Materials for Lithium‐Ion Batteries
Luo, W., Chen, X., Xia, Y., Chen, M., Wang, L., Wang, Q., Li, W., & Yang, J. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201701083 · Cited by 549
Self-citationLi, C., Li, Q., Kaneti, Y. V., Hou, D., Yamauchi, Y., & Mai, Y. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00021c · Cited by 513
New insight into the synthesis of large-pore ordered mesoporous materials
Wei, J., Sun, Z., Luo, W., Li, Y., Elzatahry, A. A., Al-Enizi, A. M., Deng, Y., & Zhao, D. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b11411 · Cited by 336
Self-citationMesoporous metallic rhodium nanoparticles
Jiang, B., Li, C., Dag, Ö., Abe, H., Takei, T., Imai, T., Hossain, M. S. A., Islam, M. T., Wood, K., Henzie, J., et al. (2017) · Nature Communications · doi:10.1038/ncomms15581 · Cited by 257
Metadata
- Authors
- Luo, W., Zhao, T., Li, Y., Wei, J., Xu, P., Li, X., Wang, Y., Zhang, W., Elzatahry, A. A., Alghamdi, A., Deng, Y., Wang, L., Jiang, W., Liu, Y., Kong, B., & Zhao, D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-09-13
- Volume
- 138
- Issue
- 38
- Pages
- 12586-12595
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2507389777
- Cited by
- 181
- References
- 2
- FWCI
- 10.82
- Type
- journal article
- Language
- en
- Open access
- green
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