The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Molecule-Level g-C3N4 Coordinated Transition Metals as a New Class of Electrocatalysts for Oxygen Electrode Reactions
Abstract
Organometallic complexes with metal–nitrogen/carbon (M–N/C) coordination are the most important alternatives to precious metal catalysts for oxygen reduction and evolution reactions (ORR and OER) in energy conversion devices. Here, we designed and developed a range of molecule-level graphitic carbon nitride (g-C 3 N 4 ) coordinated transition metals (M–C 3 N 4 ) as a new generation of M–N/C catalysts for these oxygen electrode reactions. As a proof-of-concept example, we conducted theoretical evaluation and experimental validation on a cobalt–C 3 N 4 catalyst with a desired molecular configuration, which possesses comparable electrocatalytic activity to that of precious metal benchmarks for the ORR and OER in alkaline media. The correlation of experimental and computational results confirms that this high activity originates from the precise M–N 2 coordination in the g-C 3 N 4 matrix. Moreover, the reversible ORR/OER activity trend for a wide variety of M−C 3 N 4 complexes has been constructed to provide guidance for the molecular design of this promising class of catalysts.
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Cites
A fast and robust algorithm for Bader decomposition of charge density
Henkelman, G., Arnaldsson, A., & Jónsson, H. (2006) · Computational Materials Science · doi:10.1016/j.commatsci.2005.04.010 · Cited by 10,723
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Self-citationHydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Self-citationZou, X., Huang, X., Goswami, A., Silva, R., Sathe, B. R., Mikmeková, E., & Asefa, T. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201311111 · Cited by 979
Cited by
Wan, X., Liu, X., Li, Y., Yu, R., Zheng, L., Yan, W., Wang, H., Xu, M., & Shui, J. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0237-3 · Cited by 1,379
Cao, L., Luo, Q., Liu, W., Lin, Y., Liu, X., Cao, Y., Zhang, W., Wu, Y., Yang, J., Yao, T., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0203-5 · Cited by 901
Jiang, R., Li, L., Sheng, T., Hu, G., Chen, Y., & Wang, L. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07294 · Cited by 797
Self-citationLiang, H., Gandi, A. N., Xia, C., Hedhili, M. N., Anjum, D. H., Schwingenschlögl, U., & Alshareef, H. N. (2017) · ACS Energy Letters · doi:10.1021/acsenergylett.7b00206 · Cited by 588
Zhang, H., An, P., Zhou, W., Guan, B. Y., Zhang, P., Dong, J., & Lou, X. W. (. (2018) · Science Advances · doi:10.1126/sciadv.aao6657 · Cited by 584
Metadata
- Authors
- Zheng, Y., Jiao, Y., Zhu, Y., Cai, Q., Vasileff, A., Li, L. H., Han, Y., Chen, Y., & Qiao, S.-Z.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-02-27
- Volume
- 139
- Issue
- 9
- Pages
- 3336-3339
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2591446277
- Cited by
- 1,250
- References
- 4
- FWCI
- 44.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zheng, Y., Jiao, Y., Zhu, Y., Cai, Q., Vasileff, A., Li, L. H., Han, Y., Chen, Y., & Qiao, S.-Z. (2017). Molecule-Level g-C3N4 Coordinated Transition Metals as a New Class of Electrocatalysts for Oxygen Electrode Reactions. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b13100
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