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Zn/MnO2 Battery Chemistry With H+ and Zn2+ Coinsertion
Abstract
Rechargeable aqueous Zn/MnO 2 battery chemistry in a neutral or mildly acidic electrolyte has attracted extensive attention recently because all the components (anode, cathode, and electrolyte) in a Zn/MnO 2 battery are safe, abundant, and sustainable. However, the reaction mechanism of the MnO 2 cathode remains a topic of discussion. Herein, we design a highly reversible aqueous Zn/MnO 2 battery where the binder-free MnO 2 cathode was fabricated by in situ electrodeposition of MnO 2 on carbon fiber paper in mild acidic ZnSO 4 +MnSO 4 electrolyte. Electrochemical and structural analysis identify that the MnO 2 cathode experience a consequent H + and Zn 2+ insertion/extraction process with high reversibility and cycling stability. To our best knowledge, it is the first report on rechargeable aqueous batteries with a consequent ion-insertion reaction mechanism.
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Citations
Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
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Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
Zhang, N., Dong, Y., Jia, M., Bian, X., Wang, Y., Qiu, M., Xu, J., Liu, Y., Jiao, L., & Cheng, F. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b00565 · Cited by 1,052
A Metal-Organic Framework Host for Highly Reversible Dendrite-free Zinc Metal Anodes
Wang, Z., Huang, J., Guo, Z., Dong, X., Liu, Y., Wang, Y., & Xia, Y. (2019) · Joule · doi:10.1016/j.joule.2019.02.012 · Cited by 938
Yang, Q., Liang, G., Guo, Y., Liu, Z., Yan, B., Wang, D., Huang, Z., Li, X., Fan, J., & Zhi, C. (2019) · Advanced Materials · doi:10.1002/adma.201903778 · Cited by 689
Carbon-Based Fibers for Advanced Electrochemical Energy Storage Devices
Chen, S., Qiu, L., & Cheng, H.-M. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00466 · Cited by 555
Metadata
- Authors
- Sun, W., Wang, F., Hou, S., Yang, C., Fan, X., Ma, Z., Gao, T., Han, F., Hu, R., Zhu, M., & Wang, C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-14
- Volume
- 139
- Issue
- 29
- Pages
- 9775-9778
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2735790789
- Cited by
- 1,897
- References
- 1
- FWCI
- 56.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, W., Wang, F., Hou, S., Yang, C., Fan, X., Ma, Z., Gao, T., Han, F., Hu, R., Zhu, M., & Wang, C. (2017). Zn/MnO2 Battery Chemistry With H+ and Zn2+ Coinsertion. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b04471
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