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Zn/MnO2 Battery Chemistry With H+ and Zn2+ Coinsertion
Abstract
Rechargeable aqueous Zn/MnO 2 battery chemistry in a neutral or mildly acidic electrolyte has attracted extensive attention recently because all the components (anode, cathode, and electrolyte) in a Zn/MnO 2 battery are safe, abundant, and sustainable. However, the reaction mechanism of the MnO 2 cathode remains a topic of discussion. Herein, we design a highly reversible aqueous Zn/MnO 2 battery where the binder-free MnO 2 cathode was fabricated by in situ electrodeposition of MnO 2 on carbon fiber paper in mild acidic ZnSO 4 +MnSO 4 electrolyte. Electrochemical and structural analysis identify that the MnO 2 cathode experience a consequent H + and Zn 2+ insertion/extraction process with high reversibility and cycling stability. To our best knowledge, it is the first report on rechargeable aqueous batteries with a consequent ion-insertion reaction mechanism.
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Metadata
- Authors
- Sun, W., Wang, F., Hou, S., Yang, C., Fan, X., Ma, Z., Gao, T., Han, F., Hu, R., Zhu, M., & Wang, C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-14
- Volume
- 139
- Issue
- 29
- Pages
- 9775-9778
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2735790789
- Cited by
- 1,897
- References
- 20
- FWCI
- 56.27
- Type
- journal article
- Language
- en
- Open access
- closed
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