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A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light
Abstract
Efficient and selective photostimulated CO 2 -to-CO reduction by a photocatalytic system consisting of an iron-complex catalyst and a mesoporous graphitic carbon nitride (mpg-C 3 N 4 ) redox photosensitizer is reported for the first time. Irradiation in the visible region (λ ≥ 400 nm) of an CH 3 CN/triethanolamine (4:1, v/v) solution containing [Fe(qpy)(H 2 O) 2 ] 2+ (qpy = 2,2′:6′,2′′:6′′,2′′-quaterpyridine) and mpg-C 3 N 4 resulted in CO evolution with 97% selectivity, a turnover number of 155, and an apparent quantum yield of ca. 4.2%. This hybrid catalytic system, comprising only earth abundant elements, opens new perspectives for solar fuels production using CO 2 as a renewable feedstock.
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Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Cited by
Atomic‐Level Reactive Sites for Semiconductor‐Based Photocatalytic CO2 Reduction
Zhang, Y., Xia, B., Ran, J., Davey, K., & Qiao, S. Z. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903879 · Cited by 423
Boutin, E., Merakeb, L., Ma, B., Boudy, B., Wang, M., Bonin, J., Anxolabéhère-Mallart, E., & Robert, M. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00218f · Cited by 423
Self-citationTsang, C. H. A., Li, K., Zeng, Y., Zhao, W., Zhang, T., Zhan, Y., Xie, R., Leung, D. Y. C., & Huang, H. (2019) · Environment International · doi:10.1016/j.envint.2019.01.015 · Cited by 308
Metadata
- Authors
- Cometto, C., Kuriki, R., Chen, L., Maeda, K., Lau, T.-C., Ishitani, O., & Robert, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-06-11
- Volume
- 140
- Issue
- 24
- Pages
- 7437-7440
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2808067092
- Cited by
- 214
- References
- 1
- FWCI
- 6.90
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cometto, C., Kuriki, R., Chen, L., Maeda, K., Lau, T.-C., Ishitani, O., & Robert, M. (2018). A Carbon Nitride/Fe Quaterpyridine Catalytic System for Photostimulated CO2-to-CO Conversion with Visible Light. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b04007
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