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Formation of Hierarchical Co9S8@ZnIn2S4 Heterostructured Cages as an Efficient Photocatalyst for Hydrogen Evolution
Open accessAbstract
Here we demonstrate the delicate design and construction of hierarchical Co 9 S 8 @ZnIn 2 S 4 heterostructured cages as an efficient photocatalyst for hydrogen evolution with visible light. Two photoactive sulfide semiconductors are rationally integrated into a hierarchical hollow structure with strongly coupled heterogeneous shells and two-dimensional ultrathin subunits. The unique architecture can efficiently facilitate the separation and transfer of light-induced charges, offer large surface area, and expose rich active sites for photocatalytic redox reactions. Owing to the distinctive structural and compositional benefits, the hierarchical Co 9 S 8 @ZnIn 2 S 4 hollow heterostructures without using any cocatalysts show remarkable activity with a hydrogen-producing rate of 6250 μmol h –1 g –1 and high stability for photocatalytic water splitting.
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Citations
Cited by
Qin, Y., Li, H., Lu, J., Feng, Y., Meng, F., Ma, C., Yan, Y., & Meng, M. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119254 · Cited by 518
Emerging Cocatalysts on g‐C3N4 for Photocatalytic Hydrogen Evolution
Zhu, Q., Xu, Z., Qiu, B., Xing, M., & Zhang, J. (2021) · Small · doi:10.1002/smll.202101070 · Cited by 380
Wang, Y., Wang, S., & Lou, X. W. (. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201909707 · Cited by 237
Self-citationWang, J., Yuan, L., Zhang, P., Mao, J., Fan, J., & Zhang, X. L. (2024) · Nanoscale · doi:10.1039/d3nr06411e · Cited by 21
Metadata
- Authors
- Wang, S., Guan, B. Y., Wang, X., & Lou, X. W. D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-10-31
- Volume
- 140
- Issue
- 45
- Pages
- 15145-15148
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2899228857
- Cited by
- 852
- References
- 0
- FWCI
- 19.17
- Type
- journal article
- Language
- en
- Open access
- green
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- Wang, S., Guan, B. Y., Wang, X., & Lou, X. W. D. (2018). Formation of Hierarchical Co9S8@ZnIn2S4 Heterostructured Cages as an Efficient Photocatalyst for Hydrogen Evolution. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b07721
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