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Temperature and Composition Dependence of the Density and Viscosity of Binary Mixtures of Water + Ionic Liquid
Abstract
Density and viscosity were determined for binary mixtures of water and three ionic liquids: 1-ethyl-3-methylimidazolium ethylsulfate, 1-ethyl-3-methylimidazolium trifluoroacetate, and 1-ethyl-3-methylimidazolium trifluoromethanesulfonate. The experimental measurements of these properties were carried out at atmospheric pressure and temperatures from (278.15 to 348.15) K. The temperature dependence of density and viscosity for these systems can be described by an empirical second-order polynomial and by the Vogel−Fulcher−Tammann equation, respectively. Excess molar volumes and viscosity deviations were calculated and correlated by Redlich−Kister polynomial expansions. The latter correlations describe the variation of density and viscosity with composition. Comparison of the results for the three binary systems elucidates the influence of the anion on these physical properties.
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Cites
Influence of chloride, water, and organic solvents on the physical properties of ionic liquids
Seddon, K. R., Stark, A., & Torres, M.-J. (2000) · Pure and Applied Chemistry · doi:10.1351/pac200072122275 · Cited by 2,293
Cited by
Low-transition-temperature mixtures (LTTMs): A new generation of designer solvents
Francisco, M., van den Bruinhorst, A., & Kroon, M. C. (2013) · Angewandte Chemie International Edition · doi:10.1002/anie.201207548 · Cited by 1,378
Ionic Liquids-Based Extraction: A Promising Strategy for the Advanced Nuclear Fuel Cycle
Sun, X., Luo, H., & Dai, S. (2012) · Chemical Reviews · doi:10.1021/cr200193x · Cited by 852
Goodrich, B. F., de la Fuente, J. C., Gurkan, B. E., Lopez, Z. K., Price, E. A., Huang, Y., & Brennecke, J. F. (2011) · The Journal of Physical Chemistry B · doi:10.1021/jp2015534 · Cited by 272
Self-citationLiu, F., Xue, Z., Zhao, X., Mou, H., He, J., & Mu, T. (2018) · Chemical Communications · doi:10.1039/c8cc03798a · Cited by 95
Metadata
- Authors
- Rodríguez, H., & Brennecke, J. F.
- Venue
- Journal of Chemical & Engineering Data
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-10-10
- Volume
- 51
- Issue
- 6
- Pages
- 2145-2155
- ISSN
- 0021-9568 (ISSN-L)
- 1520-5134
- OpenAlex
- W2086340877
- Cited by
- 479
- References
- 1
- FWCI
- 19.43
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rodríguez, H., & Brennecke, J. F. (2006). Temperature and Composition Dependence of the Density and Viscosity of Binary Mixtures of Water + Ionic Liquid. Journal of Chemical & Engineering Data. https://doi.org/10.1021/je0602824
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