Evaluating the performance of deep eutectic solvents for use in extractive denitrification of liquid fuels by the conductor-like screening model for real solvents
Abstract
A total of 94 deep eutectic solvents (DESs) based on different combinations of salt cation, anion, hydrogen-bond donor (HBD) and salt:HBD molar ratio are screened via the conductor-like screening model for real solvents for potential use in the extractive denitrification of diesel. Five nonbasic and six basic nitrogen compounds were included in this study. The activity coefficient at infinite dilution, γ ∞, of each nitrogen compound in the DESs was predicted; and the values are used to screen the DESs on the basis of selectivity, capacity, and performance index at infinite dilution ( S ∞, C ∞, and PI). The extraction of nitrogen compounds using DES is driven by hydrogen-bonding interaction. It was found that nonbasic compounds report higher S ∞ and C ∞ than basic compounds. Ammonium-based DESs give higher S ∞ but phosphonium-based DESs report higher C ∞ . DESs combined with Cl – anion give higher S ∞, but those with Br – anion report higher C ∞ . DESs with alcohol- and amide-based HBDs give higher S ∞ but HBDs with carboxylic acid group report high C ∞ . Molar ratio has little effect toward S ∞ and C ∞ . DESs with high values of S ∞ generally have high PI.
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Hizaddin et al. screened 94 DES using COSMO-RS and evaluated their potential usage for extractive denitrification of diesel.
“Hizaddin et al. [37] screened 94 DES by applying a conductor-like screening model for realistic solvents (COSMO-RS) and evaluated their potential usage for extractive denitrification of diesel.”
From Recent Advances in Hydrophobic Deep Eutectic Solvents for Extraction (2019) · cites this paper as [37]
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- Authors
- Hizaddin, H. F., Ramalingam, A., Hashim, M. A., & Hadj-Kali, M. K. O.
- Affiliations
- University of Malaya (MY)
- King Saud University (SA)
- Corresponding author
- Ramalingam, Anantharaj
- Venue
- Journal of Chemical & Engineering Data
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-09-18
- Volume
- 59
- Issue
- 11
- Pages
- 3470-3487
- ISSN
- 0021-9568 (ISSN-L)
- 1520-5134
- OpenAlex
- W2321777693
- Cited by
- 122
- References
- 28
- Citations by year
- 2026: 5 · 2025: 12 · 2024: 12 · 2023: 11 · 2022: 13 · 2021: 14 · 2020: 15 · 2019: 12 · 2018: 12 · 2017: 8 · 2016: 4 · 2015: 4
- FWCI
- 1.92
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Chemical & Engineering Data (publishedVersion)
- Funders
- University of Malaya (D000003-16001)
- Deanship of Scientific Research, King Saud University (RGP-VPP-108)
- Topics
- Physical Sciences › Chemical Engineering › Catalysis › Ionic liquids properties and applications
- Physical Sciences › Engineering › Mechanical Engineering › Catalysis and Hydrodesulfurization Studies
- Physical Sciences › Engineering › Biomedical Engineering › Phase Equilibria and Thermodynamics
- Keywords
- deep eutectic solvents, diesel fuel, nitrogen compound removal, infinite dilution activity coefficients, hydrogen bonding, solvent screening, performance index, basic nitrogen compounds
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