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New Metal−N−H System Composed of Mg(NH2)2 and LiH for Hydrogen Storage
Abstract
We have investigated the hydrogen storage properties of a ball-milled mixture of 3Mg(NH 2 ) 2 and 8LiH after first synthesizing Mg(NH 2 ) 2 by ball milling MgH 2 under an atmosphere of NH 3 gas at room temperature. The thermal desorption mass spectra of the mixture without any catalysts indicated that a large amount of hydrogen (∼7 wt %) was desorbed from 140 °C, and the desorption peaked at ∼190 °C under a heating rate of 5 °C/min with almost no ammonia emission. Moreover, the reversibility of the hydrogen absorption/desorption reactions was confirmed to be complete. The above results indicate that this system is one of the promising metal−N−H systems for hydrogen storage.
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Citations
Cited by
Complex Hydrides for Hydrogen Storage
Orimo, S.-I., Nakamori, Y., Eliseo, J. R., Züttel, A., & Jensen, C. M. (2007) · Chemical Reviews · doi:10.1021/cr0501846 · Cited by 2,318
(2021) · doi:10.1016/j.rser.2021.111311 · Cited by 850
Hydrogen storage: beyond conventional methods
Dalebrook, A. F., Gan, W., Grasemann, M., Moret, S., & Laurenczy, G. (2013) · Chemical Communications · doi:10.1039/c3cc43836h · Cited by 503
Hydrogen Storage Materials for Mobile and Stationary Applications: Current State of the Art
Lai, Q., Paskevicius, M., Sheppard, D. A., Buckley, C. E., Thornton, A. W., Hill, M. R., Gu, Q., Mao, J., Huang, Z., Liu, H. K., et al. (2015) · ChemSusChem · doi:10.1002/cssc.201500231 · Cited by 414
Thermodynamic and kinetic investigations of the hydrogen storage in the Li–Mg–N–H system
Xiong, Z., Hu, J., Wu, G., Chen, P., Luo, W., Gross, K., & Wang, J. (2005) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2005.02.010 · Cited by 276
Complex hydrides for energy storage, conversion, and utilization
He, T., Cao, H., & Chen, P. (2019) · Advanced Materials · doi:10.1002/adma.201902757 · Cited by 256
Metadata
- Authors
- Leng, H. Y., Ichikawa, T., Hino, S., Hanada, N., Isobe, S., & Fujii, H.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-06-09
- Volume
- 108
- Issue
- 26
- Pages
- 8763-8765
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1993683135
- Cited by
- 322
- References
- 0
- FWCI
- 18.54
- Type
- journal article
- Language
- en
- Open access
- closed
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