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Sustainable Reactions in Tunable Solvents
Abstract
There are now available a variety of tunable solvents; these have been used extensively for extractions and in a variety of materials applications. Our focus has been to apply these techniques to chemical reactions to take advantage of the special properties available, primarily for sustainable technology, to create processes that are potentially more benign and more advantageous. We report here our work in using supercritical fluids, near-critical fluids, and gas-expanded liquids to couple organic reactions with separations. In this paper, we review applications involving improved transport, catalyst recycling, and product separation as well as the in situ generation of catalysts. Although such tunable solvents are in no way a panacea, they do offer the chemical community alternatives that can often be applied creatively to many reaction opportunities.
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Cited by
The Path Forward for Biofuels and Biomaterials
Ragauskas, A. J., Williams, C. K., Davison, B. H., Britovsek, G., Cairney, J., Eckert, C. A., Frederick, W. J., Hallett, J. P., Leak, D. J., Liotta, C. L., et al. (2006) · Science · doi:10.1126/science.1114736 · Cited by 5,741
Self-citationGreen and sustainable solvents in chemical processes
Clarke, C. J., Tu, W.-C., Levers, O., Bröhl, A., & Hallett, J. P. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00571 · Cited by 2,071
Self-citationJessop, P. G., & Subramaniam, B. (2007) · Chemical Reviews · doi:10.1021/cr040199o · Cited by 561
The many faces of packed column supercritical fluid chromatography – A critical review
Lesellier, E., & West, C. (2015) · Journal of Chromatography A · doi:10.1016/j.chroma.2014.12.083 · Cited by 396
From wood to fuels: Integrating biofuels and pulp production
Ragauskas, A. J., Nagy, M., Kim, D. H., Eckert, C. A., Hallett, J. P., & Liotta, C. L. (2006) · Industrial Biotechnology · doi:10.1089/ind.2006.2.55 · Cited by 256
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Metadata
- Authors
- Eckert, C. A., Liotta, C. L., Bush, D., Brown, J. S., & Hallett, J. P.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-09-14
- Volume
- 108
- Issue
- 47
- Pages
- 18108-18118
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2165170041
- Cited by
- 162
- References
- 0
- FWCI
- 9.59
- Type
- journal article
- Language
- en
- Open access
- closed
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- Eckert, C. A., Liotta, C. L., Bush, D., Brown, J. S., & Hallett, J. P. (2004). Sustainable Reactions in Tunable Solvents. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp0487612
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
