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On the Critical Temperature, Normal Boiling Point, and Vapor Pressure of Ionic Liquids
Abstract
One-stage, reduced-pressure distillations at moderate temperature of 1-decyl- and 1-dodecyl-3-methylimidazolium bistriflilamide ([Ntf(2)](-)) ionic liquids (ILs) have been performed. These liquid-vapor equilibria can be understood in light of predictions for normal boiling points of ILs. The predictions are based on experimental surface tension and density data, which are used to estimate the critical points of several ILs and their corresponding normal boiling temperatures. In contrast to the situation found for relatively unstable ILs at high-temperature such as those containing [BF(4)](-) or [PF(6)](-) anions, [Ntf(2)](-)-based ILs constitute a promising class in which reliable, accurate vapor pressure measurements can in principle be performed. This property is paramount for assisting in the development and testing of accurate molecular models.
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Cited by
Understanding Ionic Liquids at the Molecular Level: Facts, Problems, and Controversies
Weingärtner, H. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200604951 · Cited by 1,543
State-of-the-Art of CO2Capture with Ionic Liquids
Ramdin, M., de Loos, T. W., & Vlugt, T. J. H. (2012) · Industrial & Engineering Chemistry Research · doi:10.1021/ie3003705 · Cited by 1,073
Ionic liquid thermal stabilities: decomposition mechanisms and analysis tools
Maton, C., De Vos, N., & Stevens, C. V. (2013) · Chemical Society Reviews · doi:10.1039/c3cs60071h · Cited by 889
Jin, H., O'Hare, B., Dong, J., Arzhantsev, S., Baker, G. A., Wishart, J. F., Benesi, A. J., & Maroncelli, M. (2008) · The Journal of Physical Chemistry B · doi:10.1021/jp076462h · Cited by 422
Emel'yanenko, V. N., Verevkin, S. P., & Heintz, A. (2007) · Journal of the American Chemical Society · doi:10.1021/ja0679174 · Cited by 366
Metadata
- Authors
- Rebelo, L. P. N., Canongia Lopes, J. N., Esperança, J. M. S. S., & Filipe, E.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-03-12
- Volume
- 109
- Issue
- 13
- Pages
- 6040-6043
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2012797981
- Cited by
- 516
- References
- 0
- FWCI
- 11.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rebelo, L. P. N., Canongia Lopes, J. N., Esperança, J. M. S. S., & Filipe, E. (2005). On the Critical Temperature, Normal Boiling Point, and Vapor Pressure of Ionic Liquids. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp050430h
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