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Non-Annealed Graphene Paper as a Binder-Free Anode for Lithium-Ion Batteries
Abstract
Non-annealed graphene paper, prepared via reduction of prefabricated graphene oxide paper with hydrazine hydrate, was employed as the sole component of a binder-free lithium-ion battery anode, circumventing the polymer binders and other additives required for the fabrication of conventional electrodes. The binder-free anode fabricated from this non-annealed paper possessed excellent cyclability, while exhibiting a voltage versus capacity profile similar to that of a polymer-bound graphene powder anode. Kinetic barriers may exist for Li ion diffusion through the layered paper structure as decreasing the current rate from 50 to 10 mA·g −1 increased the reversible capacity by over 150%.
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Citations
Cited by
Folded Structured Graphene Paper for High Performance Electrode Materials
Liu, F., Song, S., Xue, D., & Zhang, H. (2012) · Advanced Materials · doi:10.1002/adma.201104691 · Cited by 657
Two‐Dimensional Nanoarchitectures for Lithium Storage
Liu, J., & Liu, X. (2012) · Advanced Materials · doi:10.1002/adma.201104993 · Cited by 543
Zhao, X., Hayner, C. M., Kung, M. C., & Kung, H. H. (2011) · ACS Nano · doi:10.1021/nn202710s · Cited by 522
Chemically Active Reduced Graphene Oxide with Tunable C/O Ratios
Compton, O. C., Jain, B., Dikin, D. A., Abouimrane, A., Amine, K., & Nguyen, S. T. (2011) · ACS Nano · doi:10.1021/nn1030725 · Cited by 384
Self-citationFlexible graphene devices related to energy conversion and storage
Wang, X., & Shi, G. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03685a · Cited by 373
Metadata
- Authors
- Abouimrane, A., Compton, O. C., Amine, K., & Nguyen, S. T.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-06-30
- Volume
- 114
- Issue
- 29
- Pages
- 12800-12804
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2089465864
- Cited by
- 242
- References
- 0
- FWCI
- 17.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Abouimrane, A., Compton, O. C., Amine, K., & Nguyen, S. T. (2010). Non-Annealed Graphene Paper as a Binder-Free Anode for Lithium-Ion Batteries. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp103704y
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
