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Controllable ZnO Architectures by Ethanolamine-Assisted Hydrothermal Reaction for Enhanced Photocatalytic Activity
Abstract
Controllable ZnO architectures with different morphologies were synthesized via an ethanolamine-assisted one-pot hydrothermal method. By adjusting reaction conditions such as the molar ratio between Zn(OAc) 2 and NaOH and the volume ratio of the ethanolamine/water, the flowerlike, spindlelike, swordlike, and umbellarlike ZnO architectures of the hexagonal phase have been obtained. The as-prepared ZnO products were characterized by FE-SEM, TEM, XRD, BET, PL, and Raman spectroscopy. The ethanolamine significantly influenced the morphology of ZnO products, which is related to the competitive adsorption between ethanolamine and [Zn(OH) 4 ] 2− to ZnO nuclei. Their PL spectra depend on their morphologies and phase structures. The morphology-dependent photocatalytic performances in the degradation of methylene blue under UV illumination were observed, in which the flowerlike ZnO structures exhibit highest activity for their most irregular surface Zn sites.
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Cites
Piezoelectric Nanogenerators Based on Zinc Oxide Nanowire Arrays
Wang, Z. L., & Song, J. (2006) · Science · doi:10.1126/science.1124005 · Cited by 7,922
Flexible High-Output Nanogenerator Based on Lateral ZnO Nanowire Array
Zhu, G., Yang, R., Wang, S., & Wang, Z. L. (2010) · Nano Letters · doi:10.1021/nl101973h · Cited by 805
Cited by
Tian, C., Zhang, Q., Wu, A., Jiang, M., Liang, Z., Jiang, B., & Fu, H. (2012) · Chemical Communications · doi:10.1039/c2cc16434e · Cited by 572
Self-citationKuriakose, S., Satpati, B., & Mohapatra, S. (2014) · Physical Chemistry Chemical Physics · doi:10.1039/c4cp01315h · Cited by 364
Senapati, S., Srivastava, S. K., & Singh, S. B. (2012) · Nanoscale · doi:10.1039/c2nr31831h · Cited by 82
Metadata
- Authors
- Wang, X., Zhang, Q., Wan, Q., Dai, G., Zhou, C., & Zou, B.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-01-21
- Volume
- 115
- Issue
- 6
- Pages
- 2769-2775
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2328062150
- Cited by
- 190
- References
- 2
- FWCI
- 11.46
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, X., Zhang, Q., Wan, Q., Dai, G., Zhou, C., & Zou, B. (2011). Controllable ZnO Architectures by Ethanolamine-Assisted Hydrothermal Reaction for Enhanced Photocatalytic Activity. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp1096822
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