The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Photocatalytic Water Oxidation on BiVO4 with the Electrocatalyst as an Oxidation Cocatalyst: Essential Relations between Electrocatalyst and Photocatalyst
Abstract
The oxygen evolution is kinetically the key step in the photocatalytic water splitting. Cocatalysts could lower the activation potential for O 2 evolution. However, the cocatalyst for O 2 evolution has been less investigated, and few effective cocatalysts were reported. This paper reports that the O 2 evolution rate of photocatalytic water splitting under visible light irradiation can be significantly enhanced when the electrocatalyst cobalt–phosphate (denoted as CoPi) was deposited on BiVO 4 . The photocurrent density is also greatly enhanced by loading CoPi on BiVO 4 electrode, and this enhancement in performance shows the similar trend between the photocatalytic activity and photocurrent density. We also found that this tendency is true for BiVO 4 loaded with a series of different electrocatalysts as the cocatalysts. These results demonstrate that an effective electrocatalyst of water oxidation can be also an effective cocatalyst for O 2 evolution from photocatalytic water oxidation. By depositing the CoPi as the oxidation cocatalyst and Pt as the reduction cocatalyst on an yttrium-doped BiVO 4 (Bi 0.5 Y 0.5 VO 4 ), overall water splitting reaction to H 2 and O 2 was realized. Our work also reveals the essential relations between photocatalysis and electrocatalysis in water splitting reaction.
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Metadata
- Authors
- Wang, D., Li, R., Zhu, J., Shi, J., Han, J., Zong, X., & Li, C.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-02-22
- Volume
- 116
- Issue
- 8
- Pages
- 5082-5089
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W1970324546
- Cited by
- 379
- References
- 46
- FWCI
- 14.94
- Type
- journal article
- Language
- en
- Open access
- closed
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