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Adsorption and Separation of Xylene Isomers and Ethylbenzene on Two Zn−Terephthalate Metal−Organic Frameworks
Abstract
Metal−organic frameworks (MOFs) with metal-containing secondary building units and organic linkers have great potential for the separation of isomers. In this work, the adsorption and separation of xylene isomers and ethylbenzene (EB) on two Zn−terephthalate MOFs (MOF-5 and MOF-monoclinic) were studied by means of pulse gas chromatography, static vapor-phase adsorption, and breakthrough adsorption. The two studied Zn−terephthalate MOFs showed different selectivity and efficiency for the separation of xylene isomers and EB. On MOF-5, EB eluted first, while other isomers eluted at the same time. MOF-monoclinic showed a preferable adsorption of p -xylene over other isomers. The adsorption and separation of xylene isomers and EB were equilibrium-constant-controlled on MOF-5 and diffusion-dominated on MOF-monoclinic. On the basis of the measured McReynolds constants, MOF-5 was characterized as a stationary phase of nonpolarity, whereas MOF-monoclinic as a stationary phase of intermediate polarity for gas chromatography.
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Cites
Metal-organic frameworks with high capacity and selectivity for harmful gases
Britt, D., Tranchemontagne, D., & Yaghi, O. M. (2008) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0804900105 · Cited by 958
Cited by
Metal–Organic Frameworks for Separations
Li, J.-R., Sculley, J., & Zhou, H.-C. (2012) · Chemical Reviews · doi:10.1021/cr200190s · Cited by 6,323
Metal–Organic Frameworks for Separation
Zhao, X., Wang, Y., Li, D., Bu, X., & Feng, P. (2018) · Advanced Materials · doi:10.1002/adma.201705189 · Cited by 1,305
Yang, L., Qian, S., Wang, X., Cui, X., Chen, B., & Xing, H. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00756c · Cited by 746
Self-citationGu, Z.-Y., Yang, C.-X., Chang, N., & Yan, X.-P. (2012) · Accounts of Chemical Research · doi:10.1021/ar2002599 · Cited by 674
Self-citationMetal–Organic Frameworks for Food Safety
Wang, P.-L., Xie, L.-H., Joseph, E. A., Li, J.-R., Su, X.-O., & Zhou, H.-C. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00257 · Cited by 533
Metadata
- Authors
- Gu, Z.-Y., Jiang, D.-Q., Wang, H.-F., Cui, X.-Y., & Yan, X.-P.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-12-14
- Volume
- 114
- Issue
- 1
- Pages
- 311-316
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W1974059126
- Cited by
- 186
- References
- 1
- FWCI
- 8.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gu, Z.-Y., Jiang, D.-Q., Wang, H.-F., Cui, X.-Y., & Yan, X.-P. (2010). Adsorption and Separation of Xylene Isomers and Ethylbenzene on Two Zn−Terephthalate Metal−Organic Frameworks. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp9063017
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