The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Structure−Activity Relationship of Iron Titanate Catalysts in the Selective Catalytic Reduction of NOx with NH3
Open accessAbstract
A series of iron titanate catalysts, Fe a Ti b O x, with different Fe−Ti molar ratios are synthesized via a facile coprecipitation method and tested for the selective catalytic reduction (SCR) of NO x with NH 3 . The structural properties and redox behavior of the serial catalysts are comprehensively characterized. Comparing with pristine TiO 2 and Fe 2 O 3, the coexistence of iron and titanium species is favorable to form crystallites with specific Fe−O−Ti structure, which is highly active for the NH 3 -SCR reaction. Fe 4 Ti 4 O x catalyst with a Fe−Ti molar ratio of 1:1 shows the highest intrinsic activity, due to its smallest particle size, enhanced oxidative ability of Fe 3+, highest mobility of lattice oxygen, and abundant acid sites. The correlation between catalytic performance and reactant adsorption capability/conformation is also studied, indicating that an appropriate method to improve the low temperature SCR activity of iron titanate catalyst is to enhance the adsorption ability of NO x as monodentate nitrate on catalyst surface.
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Cites
Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Han, L., Cai, S., Gao, M., Hasegawa, J.-Y., Wang, P., Zhang, J., Shi, L., & Zhang, D. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00202 · Cited by 1,736
Metadata
- Authors
- Liu, F., & He, H.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-03-16
- Volume
- 114
- Issue
- 40
- Pages
- 16929-16936
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2168893264
- Cited by
- 350
- References
- 1
- FWCI
- 5.41
- Type
- journal article
- Language
- en
- Open access
- green
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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