The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Electrochemistry and the Future of the Automobile
Abstract
Electrification of the automobile provides a means of sustaining personal mobility in the face of petroleum resource limitations and environmental imperatives. Lithium ion (Li ion) batteries and hydrogen fuel cells provide pure-electrification solutions for different mass and usage segments of automotive application. Battery electric vehicles based on current and targeted Li ion battery technology will be limited to small-vehicle low-mileage-per-day applications; this is due to relatively low specific energy (kWh/kg) and long recharge time constraints. We briefly discuss new generations of Li ion positive and negative electrode intercalation compounds that are needed and under development to achieve energy storage density, durability, and cost targets. Lithium−air batteries give promise of extending the range, but scientists and engineers must surmount a plethora of challenges if growing research investments in this area are to prove effective. Hydrogen fuel cell vehicles have demonstrated the required ∼300 mile range and the ability to operate in all climates, but the cost of Pt-based catalysts, a low efficiency of utilization of presently cost-effective renewable sources of primary energy (e.g., electricity from wind), and the development of hydrogen infrastructure present significant challenges. Dramatic decreases in the amount of Pt used are required and are being brought to fruition along several lines of development that are described in some detail.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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Self-citationImproved Oxygen Reduction Activity on Pt 3 Ni(111) via Increased Surface Site Availability
Stamenkovic, V. R., Fowler, B., Mun, B. S., Wang, G., Ross, P. N., Lucas, C. A., & Marković, N. M. (2007) · Science · doi:10.1126/science.1135941 · Cited by 4,421
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Synthesis and Oxygen Reduction Activity of Shape-Controlled Pt3Ni Nanopolyhedra
Zhang, J., Yang, H., Fang, J., & Zou, S. (2010) · Nano Letters · doi:10.1021/nl903717z · Cited by 788
Koh, S., & Strasser, P. (2007) · Journal of the American Chemical Society · doi:10.1021/ja0742784 · Cited by 783
Truncated Octahedral Pt3Ni Oxygen Reduction Reaction Electrocatalysts
Wu, J., Zhang, J., Peng, Z., Yang, S., Wagner, F. T., & Yang, H. (2010) · Journal of the American Chemical Society · doi:10.1021/ja100571h · Cited by 520
Self-citationYano, H., Inukai, J., Uchida, H., Watanabe, M., Babu, P. K., Kobayashi, T., Chung, J. H., Oldfield, E., & Wieckowski, A. (2006) · Physical Chemistry Chemical Physics · doi:10.1039/b610573d · Cited by 187
Cited by
Electrocatalyst approaches and challenges for automotive fuel cells
Debe, M. K. (2012) · Nature · doi:10.1038/nature11115 · Cited by 5,885
Recent Advances in Electrocatalysts for Oxygen Reduction Reaction
Shao, M., Chang, Q., Dodelet, J.-P., & Chenitz, R. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00462 · Cited by 3,903
Batteries and fuel cells for emerging electric vehicle markets
Cano, Z. P., Banham, D., Ye, S., Hintennach, A., Lu, J., Fowler, M., & Chen, Z. (2018) · Nature Energy · doi:10.1038/s41560-018-0108-1 · Cited by 2,873
Recent advancements in Pt and Pt-free catalysts for oxygen reduction reaction
Nie, Y., Li, L., & Wei, Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00484a · Cited by 2,156
Kongkanand, A., & Mathias, M. F. (2016) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.6b00216 · Cited by 1,202
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Metadata
- Authors
- Wagner, F. T., Lakshmanan, B., & Mathias, M. F.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-07-06
- Volume
- 1
- Issue
- 14
- Pages
- 2204-2219
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2010814579
- Cited by
- 763
- References
- 8
- FWCI
- 47.10
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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