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Ionic Liquids for CO2 Capture and Emission Reduction
Abstract
Ionic liquids, especially those functionalized with amine groups, show significant potential for a wide variety of CO 2 separations, including postcombustion CO 2 capture. By tethering the amine to the anion, the stoichiometry of the reaction can be doubled from one CO 2 for every two amines (as is the case with aqueous monoethanolamine) to one CO 2 for each amine. Moreover, the reaction enthalpy can be actively tuned by the design of the anion, adjusting capacity and regeneration energy. In addition, ILs can be used without added water, further reducing the parasitic energy required for CO 2 removal from flue gas.
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Citations
Cited by
Carbon capture and storage (CCS): the way forward
Bui, M., Adjiman, C. S., Bardow, A., Anthony, E. J., Boston, A., Brown, S., Fennell, P. S., Fuss, S., Galindo, A., Hackett, L. A., et al. (2018) · Energy & Environmental Science · doi:10.1039/c7ee02342a · Cited by 4,374
Carbon capture and storage update
Boot-Handford, M. E., Abanades, J. C., Anthony, E. J., Blunt, M. J., Brandani, S., Mac Dowell, N., Fernández, J. R., Ferrari, M.-C., Gross, R., Hallett, J. P., et al. (2014) · Energy Environ. Sci. · doi:10.1039/c3ee42350f · Cited by 2,386
Structure and Nanostructure in Ionic Liquids
Hayes, R., Warr, G. G., & Atkin, R. (2015) · Chemical Reviews · doi:10.1021/cr500411q · Cited by 2,293
Deep Eutectic Solvents: Physicochemical Properties and Gas Separation Applications
García, G., Aparicio, S., Ullah, R., & Atilhan, M. (2015) · Energy & Fuels · doi:10.1021/ef5028873 · Cited by 1,112
State-of-the-Art of CO2Capture with Ionic Liquids
Ramdin, M., de Loos, T. W., & Vlugt, T. J. H. (2012) · Industrial & Engineering Chemistry Research · doi:10.1021/ie3003705 · Cited by 1,073
Metadata
- Authors
- Brennecke, J. F., & Gurkan, B. E.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-12-01
- Volume
- 1
- Issue
- 24
- Pages
- 3459-3464
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2555914817
- Cited by
- 547
- References
- 0
- FWCI
- 54.15
- Type
- journal article
- Language
- en
- Open access
- closed
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