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Elucidating the Photoresponse of Ultrathin MoS2 Field-Effect Transistors by Scanning Photocurrent Microscopy
Open accessAbstract
The mechanisms underlying the intrinsic photoresponse of few-layer (FL) molybdenum disulfide (MoS 2 ) field-effect transistors are investigated via scanning photocurrent microscopy. We attribute the locally enhanced photocurrent to band-bending-assisted separation of photoexcited carriers at the MoS 2 /Au interface. The wavelength-dependent photocurrents of FL MoS 2 transistors qualitatively follow the optical absorption spectra of MoS 2, providing direct evidence of interband photoexcitation. Time and spectrally resolved photocurrent measurements at varying external electric fields and carrier concentrations establish that drift-diffusion currents dominate photothermoelectric currents in devices under bias.
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Cites
Photocatalytic H2 Evolution on MoS2/CdS Catalysts under Visible Light Irradiation
Zong, X., Wu, G., Yan, H., Ma, G., Shi, J., Wen, F., Wang, L., & Li, C. (2010) · The Journal of Physical Chemistry C · doi:10.1021/jp904350e · Cited by 408
Cited by
Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides
Jariwala, D., Sangwan, V. K., Lauhon, L. J., Marks, T. J., & Hersam, M. C. (2014) · ACS Nano · doi:10.1021/nn500064s · Cited by 2,753
Self-citationPhotocurrent generation with two-dimensional van der Waals semiconductors
Buscema, M., Island, J. O., Groenendijk, D. J., Blanter, S. I., Steele, G. A., van der Zant, H. S. J., & Castellanos-Gomez, A. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00106d · Cited by 1,051
Metadata
- Authors
- Wu, C.-C., Jariwala, D., Sangwan, V. K., Marks, T. J., Hersam, M. C., & Lauhon, L. J.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-07-19
- Volume
- 4
- Issue
- 15
- Pages
- 2508-2513
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W1986326157
- Cited by
- 218
- References
- 1
- FWCI
- 11.40
- Type
- journal article
- Language
- en
- Open access
- green
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- Wu, C.-C., Jariwala, D., Sangwan, V. K., Marks, T. J., Hersam, M. C., & Lauhon, L. J. (2013). Elucidating the Photoresponse of Ultrathin MoS2 Field-Effect Transistors by Scanning Photocurrent Microscopy. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz401199x
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