The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
High-Performance Li–S Batteries with an Ultra-lightweight MWCNT-Coated Separator
Abstract
A bifunctional separator consisting of a layer of multiwall carbon nanotubes (MWCNTs) on the cathode-side of a Celgard polypropylene sheet has been investigated to overcome the challenges of Li-S cells. The conductive/porous MWCNT-coating functions (i) as an upper current collector to facilitate electron transport and high active-material utilization and (ii) as a filter to intercept/absorb the migrating polysulfides and thereby suppress the polysulfide diffusion. Also, the access to the electrolyte through the porous network of MWCNT along with its fast electronic transport facilitates the reutilization of the trapped active material and superior long-term cyclability. The MWCNT-coating is lightweight (0.17 mg cm(-2)), yet allows the successful use of regular sulfur cathodes (high sulfur content of 70 wt %) with high discharge capacity, excellent rate performance, and long cycle life, demonstrating that the MWCNT-coated separator is a viable solution to practical Li-S batteries.
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Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Cited by
Carbon materials for Li–S batteries: Functional evolution and performance improvement
Liang, J., Sun, Z.-H., Li, F., & Cheng, H.-M. (2016) · Energy Storage Materials · doi:10.1016/j.ensm.2015.09.007 · Cited by 593
Porous membranes in secondary battery technologies
Lu, W., Yuan, Z., Zhao, Y., Zhang, H., Zhang, H., & Li, X. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00823b · Cited by 479
Rational Design of Nanostructured Functional Interlayer/Separator for Advanced Li–S Batteries
Jeong, Y. C., Kim, J. H., Nam, S., Park, C. R., & Yang, S. J. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201707411 · Cited by 429
Interface engineering toward stable lithium–sulfur batteries
Guo, Y., Niu, Q., Pei, F., Wang, Q., Zhang, Y., Du, L., Zhang, Y., Zhang, Y., Zhang, Y., Fan, L., et al. (2024) · Energy & Environmental Science · doi:10.1039/d3ee04183b · Cited by 322
Gu, X., Tong, C.-J., Lai, C., Qiu, J., Huang, X., Yang, W., Wen, B., Liu, L.-M., Hou, Y., & Zhang, S. (2015) · Journal of Materials Chemistry A · doi:10.1039/c5ta04255k · Cited by 270
Metadata
- Authors
- Chung, S.-H., & Manthiram, A.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-05-22
- Volume
- 5
- Issue
- 11
- Pages
- 1978-1983
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2093803082
- Cited by
- 393
- References
- 1
- FWCI
- 22.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chung, S.-H., & Manthiram, A. (2014). High-Performance Li–S Batteries with an Ultra-lightweight MWCNT-Coated Separator. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz5006913
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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