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Hole-Conductor-Free, Metal-Electrode-Free TiO2/CH3NH3PbI3 Heterojunction Solar Cells Based on a Low-Temperature Carbon Electrode

Zhou, Huawei, Shi, Yantao, Dong, Qingshun, Zhang, Hong, Xing, Yujin, Wang, Kai, Du, Yi, Ma, Tingli·2014·The Journal of Physical Chemistry Letters

Abstract

Low cost, high efficiency, and stability are straightforward research challenges in the development of organic-inorganic perovskite solar cells. Organolead halide is unstable at high temperatures or in some solvents. The direct preparation of a carbon layer on top becomes difficult. In this study, we successfully prepared full solution-processed low-cost TiO2/CH3NH3PbI3 heterojunction (HJ) solar cells based on a low-temperature carbon electrode. Power conversion efficiency of mesoporous (M-)TiO2/CH3NH3PbI3/C HJ solar cells based on a low-temperature-processed carbon electrode achieved 9%. The devices of M-TiO2/CH3NH3PbI3/C HJ solar cells without encapsulation exhibited advantageous stability (over 2000 h) in air in the dark. The ability to process low-cost carbon electrodes at low temperature on top of the CH3NH3PbI3 layer without destroying its structure reduces the cost and simplifies the fabrication process of perovskite HJ solar cells. This ability also provides higher flexibility to choose and optimize the device, as well as investigate the underlying active layers.

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Metadata

Authors
Zhou, H., Shi, Y., Dong, Q., Zhang, H., Xing, Y., Wang, K., Du, Y., & Ma, T.
Venue
The Journal of Physical Chemistry Letters
Published
2014-09-08
Volume
5
Issue
18
Pages
3241-3246
ISSN
1948-7185 (ISSN-L)
OpenAlex
W2131232103
Cited by
290
References
2
FWCI
17.16
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Hole-Conductor-Free, Metal-Electrode-Free TiO2/CH3NH3PbI3 Heterojunction Solar Cells Based on a Low-Temperature Carbon Electrode. https://app.cochat.ai/papers/10.1021/jz5017069
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Zhou, H., Shi, Y., Dong, Q., Zhang, H., Xing, Y., Wang, K., Du, Y., & Ma, T. (2014). Hole-Conductor-Free, Metal-Electrode-Free TiO2/CH3NH3PbI3 Heterojunction Solar Cells Based on a Low-Temperature Carbon Electrode. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz5017069

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