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Tuning the Adsorption Properties of UiO-66 via Ligand Functionalization
Abstract
UiO-66 is one of the few known water-stable MOFs that are readily amenable to direct ligand substitution. In this work, UiO-66 has been synthesized with amino-, nitro-, methoxy-, and naphthyl-substituted ligands to impart polar, basic, and hydrophobic characteristics. Pure-component CO(2), CH(4), N(2), and water vapor adsorption isotherms were measured in the materials to study the effect of the functional group on the adsorption behavior. Heats of adsorption were calculated for each pure gas on each material. The results indicate that the amino-functionalized material possesses the best adsorption properties for each pure gas due to a combination of polarity and small functional group size. The naphthyl-functionalized material exhibits a good combination of inhibited water vapor adsorption and high selectivity for CO(2) over CH(4) and N(2).
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Millward, A. R., & Yaghi, O. M. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0570032 · Cited by 2,876
Cited by
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Burtch, N. C., Jasuja, H., & Walton, K. S. (2014) · Chemical Reviews · doi:10.1021/cr5002589 · Cited by 2,730
Self-citationWater adsorption in MOFs: fundamentals and applications
Canivet, J., Fateeva, A., Guo, Y., Coasne, B., & Farrusseng, D. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00078a · Cited by 1,444
Liu, X., Demir, N. K., Wu, Z., & Li, K. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b02276 · Cited by 802
Metal–Organic Frameworks for Water Harvesting from Air
Kalmutzki, M. J., Diercks, C. S., & Yaghi, O. M. (2018) · Advanced Materials · doi:10.1002/adma.201704304 · Cited by 772
Atmospheric Water Harvesting: A Review of Material and Structural Designs
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Metadata
- Authors
- Cmarik, G. E., Kim, M., Cohen, S. M., & Walton, K. S.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-10-22
- Volume
- 28
- Issue
- 44
- Pages
- 15606-15613
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W1987008661
- Cited by
- 638
- References
- 1
- FWCI
- 15.21
- Type
- journal article
- Language
- en
- Open access
- closed
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