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Super Toughened Poly(lactic acid) Ternary Blends by Simultaneous Dynamic Vulcanization and Interfacial Compatibilization
Abstract
In this study, a poly(lactic acid) (PLA) ternary blend system consisting of PLA, an epoxy-containing elastomer, and a zinc ionomer was introduced and studied in detail. Transmission electron microscopy revealed that the “salami”-like phase structure was formed in the ternary blends. While increase in blending temperature had little effects on the tensile properties of the resulting blends, it greatly changed the impact strength. For the blends prepared at 240 °C by extrusion blending, the resulting PLA ternary blends displayed supertoughness with moderate levels of strength and modulus. It was found that the zinc ions catalyzed the cross-linking of epoxy-containing elastomer and also promoted the reactive compatibilization at the interface of PLA and the elastomer. Both blending temperature and elastomer/ionomer ratio were found to play important roles in achieving supertoughness of the blends. The significant increase in notched impact strength was attributed to the effective interfacial compatibilization at elevated blending temperatures.
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Citations
Cites
A Literature Review of Poly(Lactic Acid)
Garlotta, D. (2001) · Journal of Polymers and the Environment · doi:10.1023/a:1020200822435 · Cited by 3,707
Properties of lactic acid based polymers and their correlation with composition
Södergård, A., & Stolt, M. (2002) · Progress in Polymer Science · doi:10.1016/s0079-6700(02)00012-6 · Cited by 1,461
Epoxy resins. Chemistry and technology
(1974) · International Journal of Rock Mechanics and Mining Sciences & Geomechanics Abstracts · doi:10.1016/0148-9062(74)90890-0 · Cited by 1,437
Study of Biodegradable Polylactide/Poly(butylene adipate-co-terephthalate) Blends
Jiang, L., Wolcott, M. P., & Zhang, J. (2006) · Biomacromolecules · doi:10.1021/bm050581q · Cited by 954
Self-citationAnderson, K., Schreck, K., & Hillmyer, M. (2008) · Polymer Reviews · doi:10.1080/15583720701834216 · Cited by 600
Kowalski, A., Duda, A., & Penczek, S. (2000) · Macromolecules · doi:10.1021/ma000125o · Cited by 482
Chain structure, phase morphology, and toughness relationships in polymers and blends
Wu, S. (1990) · Polymer Engineering & Science · doi:10.1002/pen.760301302 · Cited by 453
Super-tough poly(lactic acid) materials: Reactive blending with ethylene copolymer
Oyama, H. T. (2009) · Polymer · doi:10.1016/j.polymer.2008.12.025 · Cited by 393
Toughening of Polylactide by Melt Blending with a Biodegradable Poly(ether)urethane Elastomer
Li, Y., & Shimizu, H. (2007) · Macromolecular Bioscience · doi:10.1002/mabi.200700027 · Cited by 371
Toughening of polylactide by melt blending with linear low‐density polyethylene
Anderson, K. S., Lim, S. H., & Hillmyer, M. A. (2003) · Journal of Applied Polymer Science · doi:10.1002/app.12462 · Cited by 362
Dilatational bands in rubber-toughened polymers
Lazzeri, A., & Bucknall, C. B. (1993) · Journal of Materials Science · doi:10.1007/bf00356433 · Cited by 328
The effect of crosslinking on the mechanical properties of polylactic acid/polycaprolactone blends
Semba, T., Kitagawa, K., Ishiaku, U. S., & Hamada, H. (2006) · Journal of Applied Polymer Science · doi:10.1002/app.23589 · Cited by 315
Rubber toughening of polyamides with functionalized block copolymers: 1. Nylon-6
Oshinski, A. J., Keskkula, H., & Paul, D. R. (1992) · Polymer · doi:10.1016/0032-3861(92)90984-5 · Cited by 301
Anderson, K. S., & Hillmyer, M. A. (2004) · Polymer · doi:10.1016/j.polymer.2004.10.047 · Cited by 300
Li, Y., & Shimizu, H. (2009) · European Polymer Journal · doi:10.1016/j.eurpolymj.2008.12.010 · Cited by 270
Toughening modification of PLLA/PBS blends via in situ compatibilization
Wang, R., Wang, S., Zhang, Y., Wan, C., & Ma, P. (2009) · Polymer Engineering & Science · doi:10.1002/pen.21210 · Cited by 266
Surprising shape-memory effect of polylactide resulted from toughening by polyamide elastomer
Zhang, W., Chen, L., & Zhang, Y. (2009) · Polymer · doi:10.1016/j.polymer.2009.01.032 · Cited by 245
Kim, G.-E., & Michler, G. H. (1998) · Polymer · doi:10.1016/s0032-3861(98)00089-5 · Cited by 242
Characterisation of multi-extruded poly(lactic acid)
Żenkiewicz, M., Richert, J., Rytlewski, P., Moraczewski, K., Stepczyńska, M., & Karasiewicz, T. (2009) · Polymer Testing · doi:10.1016/j.polymertesting.2009.01.012 · Cited by 241
Zhang, N., Wang, Q., Ren, J., & Wang, L. (2009) · Journal of Materials Science · doi:10.1007/s10853-008-3049-4 · Cited by 240
Polymer Alloys of Nodax Copolymers and Poly(lactic acid)
Noda, I., Satkowski, M. M., Dowrey, A. E., & Marcott, C. (2004) · Macromolecular Bioscience · doi:10.1002/mabi.200300093 · Cited by 214
Su, Z., Li, Q., Liu, Y., Hu, G.-H., & Wu, C. (2009) · European Polymer Journal · doi:10.1016/j.eurpolymj.2009.04.028 · Cited by 203
Influence of processing parameters on the degradation of poly( L ‐lactide) during extrusion
Taubner, V., & Shishoo, R. (2001) · Journal of Applied Polymer Science · doi:10.1002/1097-4628(20010321)79:12<2128::aid-app1020>3.0.co;2-# · Cited by 199
On the role of intermolecular hydrogen bonding in miscible polymer blends
Moskala, E. J., Howe, S. E., Painter, P. C., & Coleman, M. M. (1984) · Macromolecules · doi:10.1021/ma00139a006 · Cited by 198
Craze initiation and growth in high‐impact polystyrene
Donald, A. M., & Krämer, E. J. (1982) · Journal of Applied Polymer Science · doi:10.1002/app.1982.070271009 · Cited by 196
Dompas, D., & Groeninckx, G. (1994) · Polymer · doi:10.1016/0032-3861(94)90727-7 · Cited by 192
Ho, C.-H., Wang, C.-H., Lin, C.-I., & Lee, Y.-D. (2008) · Polymer · doi:10.1016/j.polymer.2008.06.054 · Cited by 190
Thermal properties and physical ageing of poly (l-lactic acid)
Celli, A., & Scandola, M. (1992) · Polymer · doi:10.1016/0032-3861(92)90440-8 · Cited by 188
Modification of Brittle Polylactide by Novel Hyperbranched Polymer-Based Nanostructures
Bhardwaj, R., & Mohanty, A. K. (2007) · Biomacromolecules · doi:10.1021/bm070367x · Cited by 185
Toughening of Polylactide with Polymerized Soybean Oil
Robertson, M. L., Chang, K., Gramlich, W. M., & Hillmyer, M. A. (2010) · Macromolecules · doi:10.1021/ma9022795 · Cited by 161
Huang, J., Keskkula, H., & Paul, D. R. (2005) · Polymer · doi:10.1016/j.polymer.2005.11.088 · Cited by 123
Acid salts and the structure of ionomers
Coleman, M. M., Lee, J. Y., & Painter, P. C. (1990) · Macromolecules · doi:10.1021/ma00210a033 · Cited by 109
Oshinski, A. J., Keskkula, H., & Paul, D. R. (1996) · Polymer · doi:10.1016/0032-3861(96)00374-6 · Cited by 109
Dompas, D., Groeninckx, G., Isogawa, M., Hasegawa, T., & Kadokura, M. (1994) · Polymer · doi:10.1016/0032-3861(94)90728-5 · Cited by 90
Schreck, K. M., & Hillmyer, M. A. (2007) · Journal of Biotechnology · doi:10.1016/j.jbiotec.2007.03.017 · Cited by 88
Cho, K., Yang, J., & Park, C. E. (1998) · Polymer · doi:10.1016/s0032-3861(97)10036-2 · Cited by 82
Internal structure of rubber particles and craze break-down in high-impact polystyrene (HIPS)
Donald, A. M., & Kramer, E. J. (1982) · Journal of Materials Science · doi:10.1007/bf00543744 · Cited by 76
Oshinski, A. J., Keskkula, H., & Paul, D. R. (1996) · Journal of Applied Polymer Science · Cited by 60
Cho, K., Yang, J., & Park, C. E. (1997) · Polymer · doi:10.1016/s0032-3861(97)00052-9 · Cited by 54
Takaki, A., Yasui, H., & Narisawa, I. (1997) · Polymer Engineering and Science · doi:10.1002/pen.11651 · Cited by 44
Cigna, G., Lomellini, P., & Merlotti, M. (1989) · Journal of Applied Polymer Science · doi:10.1002/app.1989.070370607 · Cited by 34
Do, H., Park, J., & Kim, H. (2008) · Journal of Applied Polymer Science · doi:10.1002/app.28954 · Cited by 34
Perego (1998) · doi:10.1002/(sici)1097-4628(19960103)59:1<37::aid-app6>3.0.co;2-n
Cited by
Nagarajan, V., Mohanty, A. K., & Misra, M. (2016) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.6b00321 · Cited by 926
Poly (lactic acid) blends: Processing, properties and applications
Nofar, M., Sacligil, D., Carreau, P. J., Kamal, M. R., & Heuzey, M.-C. (2019) · International Journal of Biological Macromolecules · doi:10.1016/j.ijbiomac.2018.12.002 · Cited by 780
Research progress in toughening modification of poly(lactic acid)
Liu, H., & Zhang, J. (2011) · Journal of Polymer Science Part B: Polymer Physics · doi:10.1002/polb.22283 · Cited by 767
Self-citationControlled Polymerization of Next-Generation Renewable Monomers and Beyond
Yao, K., & Tang, C. (2013) · Macromolecules · doi:10.1021/ma3019574 · Cited by 485
Super tough poly(lactic acid) blends: a comprehensive review
Zhao, X., Hu, H., Wang, X., Yu, X., Zhou, W., & Peng, S. (2020) · RSC Advances · doi:10.1039/d0ra01801e · Cited by 465
Metadata
- Authors
- Liu, H., Chen, F., Liu, B., Estep, G., & Zhang, J.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-06-30
- Volume
- 43
- Issue
- 14
- Pages
- 6058-6066
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2095244878
- Cited by
- 323
- References
- 43
- FWCI
- 13.61
- Type
- journal article
- Language
- en
- Open access
- closed
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