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σ Phase Formed in Conformationally Asymmetric AB-Type Block Copolymers
Abstract
The stability of various spherical phases formed in conformationally asymmetric AB diblock and architecture asymmetric AB m miktoarm block copolymers is investigated using self-consistent field theory. Both the conformational and architecture asymmetries are unified into a parameter of conformationally asymmetric degree, ε. We find that a complex spherical phase, the σ phase, becomes stable and its phase region expands between bcc and hexagonal phases as increasing ε. Only for large conformational asymmetry, for example, ε = 9 (or m = 3), the A15 phase becomes stable in the region between the σ phase and the hexagonal phase and its phase region terminates at the intermediate segregation region. Compared with the σ phase, the A15 phase has more favorable interfacial energy by enabling the formation of larger spherical domains, and therefore, it becomes more stable in the region of more symmetric volume fraction and stronger segregation.
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Citations
Cites
Fluctuations, Order, and Disorder in Short Diblock Copolymers
Lee, S., Gillard, T. M., & Bates, F. S. (2013) · AIChE Journal · doi:10.1002/aic.14023 · Cited by 100
Cited by
50th Anniversary Perspective: Block Polymers—Pure Potential
Bates, C. M., & Bates, F. S. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02355 · Cited by 788
Thermal processing of diblock copolymer melts mimics metallurgy
Kim, K., Schulze, M. W., Arora, A., Lewis, R. M., Hillmyer, M. A., Dorfman, K. D., & Bates, F. S. (2017) · Science · doi:10.1126/science.aam7212 · Cited by 295
Metadata
- Authors
- Xie, N., Li, W., Qiu, F., & Shi, A.-C.
- Venue
- ACS Macro Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-09-02
- Volume
- 3
- Issue
- 9
- Pages
- 906-910
- ISSN
- 2161-1653 (ISSN-L)
- OpenAlex
- W2322734859
- Cited by
- 287
- References
- 1
- FWCI
- 6.40
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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