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Effect of Processing Additive on the Nanomorphology of a Bulk Heterojunction Material
Abstract
The bulk heterojunction (BHJ) material Si-PDTBT:PC(70)BM is sensitive to the use of a small amount of 1-chloronaphthalene (CN) as a processing additive; CN as a cosolvent (e.g., 4% in chlorobenzene) causes in a factor of 2 increase in the power conversion efficiency of BHJ solar cells. The morphology of the BHJ material, prepared with and without the CN additive is studied with top-down transmission electron microscopy, cross-sectional transmission electron microscopy, and atomic force microscopy. The improved performance is the result of changes in the nanoscale morphology. Field-effect transistor measurements are consistent with the observed changes in morphology.
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Citations
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Coffin, R. C., Peet, J., Rogers, J., & Bazan, G. C. (2009) · Nature Chemistry · doi:10.1038/nchem.403 · Cited by 597
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Cited by
Bulk Heterojunction Solar Cells: Morphology and Performance Relationships
Huang, Y., Kramer, E. J., Heeger, A. J., & Bazan, G. C. (2014) · Chemical Reviews · doi:10.1021/cr400353v · Cited by 1,249
Self-citationBulk‐Heterojunction Organic Solar Cells: Five Core Technologies for Their Commercialization
Kang, H., Kim, G., Kim, J., Kwon, S., Kim, H., & Lee, K. (2016) · Advanced Materials · doi:10.1002/adma.201601197 · Cited by 489
Self-citationSmall is Powerful: Recent Progress in Solution‐Processed Small Molecule Solar Cells
Collins, S. D., Ran, N. A., Heiber, M. C., & Nguyen, T. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201602242 · Cited by 414
Recent progress in organic photovoltaics: device architecture and optical design
Cao, W., & Xue, J. (2014) · Energy & Environmental Science · doi:10.1039/c4ee00260a · Cited by 356
Bian, L., Zhu, E., Tang, J., Tang, W., & Zhang, F. (2012) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2012.03.001 · Cited by 269
Metadata
- Authors
- Moon, J. S., Takacs, C. J., Cho, S., Coffin, R. C., Kim, H., Bazan, G. C., & Heeger, A. J.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-09-08
- Volume
- 10
- Issue
- 10
- Pages
- 4005-4008
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W1988116333
- Cited by
- 238
- References
- 1
- FWCI
- 21.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Moon, J. S., Takacs, C. J., Cho, S., Coffin, R. C., Kim, H., Bazan, G. C., & Heeger, A. J. (2010). Effect of Processing Additive on the Nanomorphology of a Bulk Heterojunction Material. Nano Letters. https://doi.org/10.1021/nl101923m
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
