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On the Energy Shift between Near-Field and Far-Field Peak Intensities in Localized Plasmon Systems
Abstract
The localized plasmons of metallic nanoparticles and nanostructures are known to display an interesting and apparently universal phenomenon: upon optical excitation, the maximum near-field enhancements occur at lower energies than the maximum of the corresponding far-field spectrum. Here we present an explanation for this behavior, showing that it results directly from the physics of a driven and damped harmonic oscillator. We show that the magnitude of the shift between the near- and far-field peak intensities depends directly on the total damping of the system, whether it is intrinsic damping within the metal of the nanoparticle or radiative damping of the localized plasmon.
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Cited by
Single-Molecule Plasmon Sensing: Current Status and Future Prospects
Taylor, A. B., & Zijlstra, P. (2017) · ACS Sensors · doi:10.1021/acssensors.7b00382 · Cited by 366
Molecular cavity optomechanics as a theory of plasmon-enhanced Raman scattering
Roelli, P., Galland, C., Piro, N., & Kippenberg, T. J. (2016) · Nature Nanotechnology · doi:10.1038/nnano.2015.264 · Cited by 276
Surface-Enhanced Infrared Spectroscopy Using Nanometer-Sized Gaps
Huck, C., Neubrech, F., Vogt, J., Toma, A., Gerbert, D., Katzmann, J., Härtling, T., & Pucci, A. (2014) · ACS Nano · doi:10.1021/nn500903v · Cited by 225
Knight, M. W., Coenen, T., Yang, Y., Brenny, B. J. M., Losurdo, M., Brown, A. S., Everitt, H. O., & Polman, A. (2015) · ACS Nano · doi:10.1021/nn5072254 · Cited by 174
Self-Similar Multiresonant Nanoantenna Arrays for Sensing from Near- to Mid-Infrared
Rodrigo, D., Tittl, A., John-Herpin, A., Limaj, O., & Altug, H. (2018) · ACS Photonics · doi:10.1021/acsphotonics.8b01050 · Cited by 85
Metadata
- Authors
- Zuloaga, J., & Nordlander, P.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-02-14
- Volume
- 11
- Issue
- 3
- Pages
- 1280-1283
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2089493917
- Cited by
- 371
- References
- 0
- FWCI
- 17.69
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
