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Hollow Iron Oxide Nanoparticles for Application in Lithium Ion Batteries
Abstract
Material design in terms of their morphologies other than solid nanoparticles can lead to more advanced properties. At the example of iron oxide, we explored the electrochemical properties of hollow nanoparticles with an application as a cathode and anode. Such nanoparticles contain very high concentration of cation vacancies that can be efficiently utilized for reversible Li ion intercalation without structural change. Cycling in high voltage range results in high capacity (∼132 mAh/g at 2.5 V), 99.7% Coulombic efficiency, superior rate performance (133 mAh/g at 3000 mA/g) and excellent stability (no fading at fast rate during more than 500 cycles). Cation vacancies in hollow iron oxide nanoparticles are also found to be responsible for the enhanced capacity in the conversion reactions. We monitored in situ structural transformation of hollow iron oxide nanoparticles by synchrotron X-ray absorption and diffraction techniques that provided us clear understanding of the lithium intercalation processes during electrochemical cycling.
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Cited by
Review on recent progress of nanostructured anode materials for Li-ion batteries
Goriparti, S., Miele, E., De Angelis, F., Di Fabrizio, E., Proietti Zaccaria, R., & Capiglia, C. (2014) · Journal of Power Sources · doi:10.1016/j.jpowsour.2013.11.103 · Cited by 2,092
Synthesis, Properties, and Applications of Hollow Micro-/Nanostructures
Wang, X., Feng, J., Bai, Y., Zhang, Q., & Yin, Y. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00731 · Cited by 1,456
Defect Engineering on Electrode Materials for Rechargeable Batteries
Zhang, Y., Tao, L., Xie, C., Wang, D., Zou, Y., Chen, R., Wang, Y., Jia, C., & Wang, S. (2020) · Advanced Materials · doi:10.1002/adma.201905923 · Cited by 1,019
Electrode Degradation in Lithium-Ion Batteries
Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Luo, J., Liu, J., Zeng, Z., Ng, C. F., Ma, L., Zhang, H., Lin, J., Shen, Z., & Fan, H. J. (2013) · Nano Letters · doi:10.1021/nl403461n · Cited by 773
Metadata
- Authors
- Koo, B., Xiong, H., Slater, M. D., Prakapenka, V. B., Balasubramanian, M., Podsiadlo, P., Johnson, C. S., Rajh, T., & Shevchenko, E. V.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-04-11
- Volume
- 12
- Issue
- 5
- Pages
- 2429-2435
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2044790533
- Cited by
- 407
- References
- 0
- FWCI
- 35.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Koo, B., Xiong, H., Slater, M. D., Prakapenka, V. B., Balasubramanian, M., Podsiadlo, P., Johnson, C. S., Rajh, T., & Shevchenko, E. V. (2012). Hollow Iron Oxide Nanoparticles for Application in Lithium Ion Batteries. Nano Letters. https://doi.org/10.1021/nl3004286
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