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Synthesis of Patched or Stacked Graphene and hBN Flakes: A Route to Hybrid Structure Discovery
Abstract
Two-dimensional (2D) materials such as graphene and hexagonal boron nitride (hBN) have attracted significant attention due to their remarkable properties. Numerous interesting graphene/hBN hybrid structures have been proposed but their implementation has been very limited. In this work, the synthesis of patched structures through consecutive chemical vapor deposition (CVD) on the same substrate was investigated. Both in-plane junctions and stacked layers were obtained. For stacked layers, depending on the synthesis sequence, in one case turbostratic stacking with random rotations were obtained. In another, "AA-like", slightly twisted stacking between graphene and hBN was observed with lattice orientation misalignment consistently to be <1°. Raman characterizations not only confirmed that hBN is a superior substrate but also revealed for the first time that a graphene edge with hBN passivation displays reduced D band intensity compared to an open edge. These studies pave the way for the proposed well-ordered graphene/hBN structures and outline exciting future directions for hybrid 2D materials.
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Cites
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Fine Structure Constant Defines Visual Transparency of Graphene
Nair, R. R., Blake, P., Grigorenko, A. N., Novoselov, K. S., Booth, T. J., Stauber, T., Peres, N. M. R., & Geim, A. K. (2008) · Science · doi:10.1126/science.1156965 · Cited by 9,084
Cited by
Science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems
Ferrari, A. C., Bonaccorso, F., Fal'ko, V., Novoselov, K. S., Roche, S., Bøggild, P., Borini, S., Koppens, F. H. L., Palermo, V., Pugno, N., et al. (2015) · Nanoscale · doi:10.1039/c4nr01600a · Cited by 3,027
Rise of silicene: A competitive 2D material
Zhao, J., Liu, H., Yu, Z., Quhe, R., Zhou, S., Wang, Y., Liu, C. C., Zhong, H., Han, N., Lu, J., et al. (2016) · Progress in Materials Science · doi:10.1016/j.pmatsci.2016.04.001 · Cited by 891
Two-dimensional heterostructures: fabrication, characterization, and application
Wang, H., Liu, F., Fu, W., Fang, Z., Zhou, W., & Liu, Z. (2014) · Nanoscale · doi:10.1039/c4nr03435j · Cited by 403
Synthesis, structure and applications of graphene-based 2D heterostructures
Solís-Fernández, P., Bissett, M., & Ago, H. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00160f · Cited by 371
Auwärter, W. (2019) · Surface Science Reports · doi:10.1016/j.surfrep.2018.10.001 · Cited by 264
Metadata
- Authors
- Kim, S. M., Hsu, A., Araujo, P. T., Lee, Y.-H., Palacios, T., Dresselhaus, M., Idrobo, J.-C., Kim, K. K., & Kong, J.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-03-04
- Volume
- 13
- Issue
- 3
- Pages
- 933-941
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2312857983
- Cited by
- 201
- References
- 2
- FWCI
- 10.80
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kim, S. M., Hsu, A., Araujo, P. T., Lee, Y.-H., Palacios, T., Dresselhaus, M., Idrobo, J.-C., Kim, K. K., & Kong, J. (2013). Synthesis of Patched or Stacked Graphene and hBN Flakes: A Route to Hybrid Structure Discovery. Nano Letters. https://doi.org/10.1021/nl303760m
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