The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
A Fully Integrated Nanosystem of Semiconductor Nanowires for Direct Solar Water Splitting
Open accessAbstract
Artificial photosynthesis, the biomimetic approach to converting sunlight's energy directly into chemical fuels, aims to imitate nature by using an integrated system of nanostructures, each of which plays a specific role in the sunlight-to-fuel conversion process. Here we describe a fully integrated system of nanoscale photoelectrodes assembled from inorganic nanowires for direct solar water splitting. Similar to the photosynthetic system in a chloroplast, the artificial photosynthetic system comprises two semiconductor light absorbers with large surface area, an interfacial layer for charge transport, and spatially separated cocatalysts to facilitate the water reduction and oxidation. Under simulated sunlight, a 0.12% solar-to-fuel conversion efficiency is achieved, which is comparable to that of natural photosynthesis. The result demonstrates the possibility of integrating material components into a functional system that mimics the nanoscopic integration in chloroplasts. It also provides a conceptual blueprint of modular design that allows incorporation of newly discovered components for improved performance.
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Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
Photocatalytic Water Splitting: Recent Progress and Future Challenges
Maeda, K., & Domen, K. (2010) · The Journal of Physical Chemistry Letters · doi:10.1021/jz1007966 · Cited by 2,739
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
Comparing Photosynthetic and Photovoltaic Efficiencies and Recognizing the Potential for Improvement
Blankenship, R. E., Tiede, D. M., Barber, J., Brudvig, G. W., Fleming, G., Ghirardi, M., Gunner, M. R., Junge, W., Kramer, D. M., Melis, A., et al. (2011) · Science · doi:10.1126/science.1200165 · Cited by 1,638
Cited by
Kong, D., Wang, H., Lu, Z., & Cui, Y. (2014) · Journal of the American Chemical Society · doi:10.1021/ja501497n · Cited by 1,392
A Review of Direct Z‐Scheme Photocatalysts
Low, J., Jiang, C., Cheng, B., Wageh, S., Al‐Ghamdi, A. A., & Yu, J. (2017) · Small Methods · doi:10.1002/smtd.201700080 · Cited by 1,381
Wang, H., Lee, H.-W., Deng, Y., Lu, Z., Hsu, P.-C., Liu, Y., Lin, D., & Cui, Y. (2015) · Nature Communications · doi:10.1038/ncomms8261 · Cited by 1,257
Yeh, T., Teng, C., Chen, S., & Teng, H. (2014) · Advanced Materials · doi:10.1002/adma.201305299 · Cited by 873
Efficient solar water-splitting using a nanocrystalline CoO photocatalyst
Liao, L., Zhang, Q., Su, Z., Zhao, Z., Wang, Y., Li, Y., Lu, X., Wei, D., Feng, G., Yu, Q., et al. (2014) · Nature Nanotechnology · doi:10.1038/nnano.2013.272 · Cited by 852
Metadata
- Authors
- Liu, C., Tang, J., Chen, H. M., Liu, B., & Yang, P.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-05-06
- Volume
- 13
- Issue
- 6
- Pages
- 2989-2992
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2178973010
- Cited by
- 549
- References
- 4
- FWCI
- 27.53
- Type
- journal article
- Language
- en
- Open access
- green
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- Liu, C., Tang, J., Chen, H. M., Liu, B., & Yang, P. (2013). A Fully Integrated Nanosystem of Semiconductor Nanowires for Direct Solar Water Splitting. Nano Letters. https://doi.org/10.1021/nl401615t
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