The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Atomistic Origins of High Rate Capability and Capacity of N-Doped Graphene for Lithium Storage
Abstract
Distinct from pure graphene, N-doped graphene (GN) has been found to possess high rate capability and capacity for lithium storage. However, there has still been a lack of direct experimental evidence and fundamental understanding of the storage mechanisms at the atomic scale, which may shed a new light on the reasons of the ultrafast lithium storage property and high capacity for GN. Here we report on the atomistic insights of the GN energy storage as revealed by in situ transmission electron microscopy (TEM). The lithiation process on edges and basal planes is directly visualized, the pyrrolic N "hole" defect and the perturbed solid-electrolyte-interface configurations are observed, and charge transfer states for three N-existing forms are also investigated. In situ high-resolution TEM experiments together with theoretical calculations provide a solid evidence that enlarged edge {0002} spacings and surface hole defects result in improved surface capacitive effects and thus high rate capability and the high capacity are owing to short-distance orderings at the edges during discharging and numerous surface defects; the phenomena cannot be understood previously by standard electron or X-ray diffraction analyses.
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1 retracted
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Self-citationGraphene‐Based Materials: Synthesis, Characterization, Properties, and Applications
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Cited by
Li, Y., Xiao, K., Huang, C., Wang, J., Gao, M., Hu, A., Tang, Q., Fan, B., Xu, Y., & Chen, X. (2021) · Nano-Micro Letters · doi:10.1007/s40820-020-00525-y · Cited by 892
Porous Carbons: Structure‐Oriented Design and Versatile Applications
Tian, W., Zhang, H., Duan, X., Sun, H., Shao, G., & Wang, S. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201909265 · Cited by 657
Self-citationHeteroatom-doped carbon-based materials for lithium and sodium ion batteries
Yuan, Y., Chen, Z., Yu, H., Zhang, X., Liu, T., Xia, M., Zheng, R., Shui, M., & Shu, J. (2020) · Energy Storage Materials · doi:10.1016/j.ensm.2020.07.027 · Cited by 455
Synthesis, properties and applications of graphene doped with boron, nitrogen and other elements
Rao, C. N. R., Gopalakrishnan, K., & Govindaraj, A. (2014) · Nano Today · doi:10.1016/j.nantod.2014.04.010 · Cited by 450
Synthesis and applications of MOF-derived porous nanostructures
Yap, M. H., Fow, K. L., & Chen, G. Z. (2017) · Green Energy & Environment · doi:10.1016/j.gee.2017.05.003 · Cited by 441
Metadata
- Authors
- Wang, X., Weng, Q., Liu, X., Wang, X., Tang, D.-M., Tian, W., Zhang, C., Yi, W., Liu, D., Bando, Y., & Golberg, D.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-02-05
- Volume
- 14
- Issue
- 3
- Pages
- 1164-1171
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2320634911
- Cited by
- 320
- References
- 46
- FWCI
- 22.29
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, X., Weng, Q., Liu, X., Wang, X., Tang, D.-M., Tian, W., Zhang, C., Yi, W., Liu, D., Bando, Y., & Golberg, D. (2014). Atomistic Origins of High Rate Capability and Capacity of N-Doped Graphene for Lithium Storage. Nano Letters. https://doi.org/10.1021/nl4038592
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