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Engineering Light Outcoupling in 2D Materials
Abstract
When light is incident on 2D transition metal dichalcogenides (TMDCs), it engages in multiple reflections within underlying substrates, producing interferences that lead to enhancement or attenuation of the incoming and outgoing strength of light. Here, we report a simple method to engineer the light outcoupling in semiconducting TMDCs by modulating their dielectric surroundings. We show that by modulating the thicknesses of underlying substrates and capping layers, the interference caused by substrate can significantly enhance the light absorption and emission of WSe2, resulting in a ∼11 times increase in Raman signal and a ∼30 times increase in the photoluminescence (PL) intensity of WSe2. On the basis of the interference model, we also propose a strategy to control the photonic and optoelectronic properties of thin-layer WSe2. This work demonstrates the utilization of outcoupling engineering in 2D materials and offers a new route toward the realization of novel optoelectronic devices, such as 2D LEDs and solar cells.
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Cited by
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Li, H., Contryman, A. W., Qian, X., Ardakani, S. M., Gong, Y., Wang, X., Weisse, J. M., Lee, C. H., Zhao, J., Ajayan, P. M., et al. (2015) · Nature Communications · doi:10.1038/ncomms8381 · Cited by 478
Wang, J., Fang, H., Wang, X., Chen, X., Lu, W., & Hu, W. (2017) · Small · doi:10.1002/smll.201700894 · Cited by 339
Amani, M., Taheri, P., Addou, R., Ahn, G. H., Kiriya, D., Lien, D.-H., Ager, J. W., Wallace, R. M., & Javey, A. (2016) · Nano Letters · doi:10.1021/acs.nanolett.6b00536 · Cited by 294
Self-citationHigh temperature thermal management with boron nitride nanosheets
Wang, Y., Xu, L., Yang, Z., Xie, H., Jiang, P., Dai, J., Luo, W., Yao, Y., Hitz, E., Yang, R., et al. (2018) · Nanoscale · doi:10.1039/c7nr07058f · Cited by 66
Metadata
- Authors
- Lien, D.-H., Kang, J. S., Amani, M., Chen, K., Tosun, M., Wang, H.-P., Roy, T., Eggleston, M. S., Wu, M. C., Dubey, M., Lee, S.-C., He, J.-H., & Javey, A.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-01-26
- Volume
- 15
- Issue
- 2
- Pages
- 1356-1361
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W1990770183
- Cited by
- 166
- References
- 0
- FWCI
- 8.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lien, D.-H., Kang, J. S., Amani, M., Chen, K., Tosun, M., Wang, H.-P., Roy, T., Eggleston, M. S., Wu, M. C., Dubey, M., Lee, S.-C., He, J.-H., & Javey, A. (2015). Engineering Light Outcoupling in 2D Materials. Nano Letters. https://doi.org/10.1021/nl504632u
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