The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
The Role of Intercalated Water in Multilayered Graphene Oxide
Abstract
A detailed in situ infrared spectroscopy analysis of single layer and multilayered graphene oxide (GO) thin films reveals that the normalized infrared absorption in the carbonyl region is substantially higher in multilayered GO upon mild annealing. These results highlight the fact that the reduction chemistry of multilayered GO is dramatically different from the single layer GO due to the presence of water molecules confined in the ∼1 nm spacing between sheets. IR spectroscopy, XPS analysis, and DFT calculations all confirm that the water molecules play a significant role interacting with basal plane etch holes through passivation, via evolution of CO(2) leading to the formation of ketone and ester carbonyl groups. Displacement of water from intersheet spacing with alcohol significantly changes the chemistry of carbonyl formation with temperature.
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Citations
Cites
Projector augmented-wave method
Blöchl, P. E. (1994) · Physical Review B · doi:10.1103/physrevb.50.17953 · Cited by 92,732
The chemistry of graphene oxide
Dreyer, D. R., Park, S., Bielawski, C. W., & Ruoff, R. S. (2010) · Chem. Soc. Rev. · doi:10.1039/b917103g · Cited by 11,653
Cited by
Acik, M., Lee, G., Mattevi, C., Pirkle, A., Wallace, R. M., Chhowalla, M., Cho, K., & Chabal, Y. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp2052618 · Cited by 961
Self-citationGraphene and graphene oxide as nanomaterials for medicine and biology application
Priyadarsini, S., Mohanty, S., Mukherjee, S., Basu, S., & Mishra, M. (2018) · Journal of Nanostructure in Chemistry · doi:10.1007/s40097-018-0265-6 · Cited by 570
Graphene oxide and its reduction: modeling and experimental progress
Mao, S., Pu, H., & Chen, J. (2012) · RSC Advances · doi:10.1039/c2ra00663d · Cited by 522
The Chemistry of Graphene Oxide
Gao, W. (2015) · Graphene Oxide · doi:10.1007/978-3-319-15500-5_3 · Cited by 459
Restacking-Inhibited 3D Reduced Graphene Oxide for High Performance Supercapacitor Electrodes
Lee, J. H., Park, N., Kim, B. G., Jung, D. S., Im, K., Hur, J., & Choi, J. W. (2013) · ACS Nano · doi:10.1021/nn4040734 · Cited by 425
Metadata
- Authors
- Acik, M., Mattevi, C., Gong, C., Lee, G., Cho, K., Chhowalla, M., & Chabal, Y. J.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-10-01
- Volume
- 4
- Issue
- 10
- Pages
- 5861-5868
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2329950272
- Cited by
- 424
- References
- 2
- FWCI
- 11.89
- Type
- journal article
- Language
- en
- Open access
- closed
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