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Electrochemistry of Individual Monolayer Graphene Sheets
Abstract
We report on the fabrication and measurement of devices designed to study the electrochemical behavior of individual monolayer graphene sheets as electrodes. We have examined both mechanically exfoliated and chemical vapor deposited (CVD) graphene. The effective device areas, determined from cyclic voltammetric measurements, show good agreement with the geometric area of the graphene sheets, indicating that the redox reactions occur on clean graphene surfaces. The electron transfer rates of ferrocenemethanol at both types of graphene electrodes were found to be more than 10-fold faster than at the basal plane of bulk graphite, which we ascribe to corrugations in the graphene sheets. We further describe an electrochemical investigation of adsorptive phenomena on graphene surfaces. Our results show that electrochemistry can provide a powerful means of investigating the interactions between molecules and the surfaces of graphene sheets as electrodes.
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Citations
Cites
Graphene: Status and Prospects
Geim, A. K. (2009) · Science · doi:10.1126/science.1158877 · Cited by 13,942
Cited by
Electrochemistry of Graphene and Related Materials
Ambrosi, A., Chua, C. K., Bonanni, A., & Pumera, M. (2014) · Chemical Reviews · doi:10.1021/cr500023c · Cited by 1,208
The edge- and basal-plane-specific electrochemistry of a single-layer graphene sheet
Yuan, W., Zhou, Y., Li, Y., Li, C., Peng, H., Zhang, J., Liu, Z., Dai, L., & Shi, G. (2013) · Scientific Reports · doi:10.1038/srep02248 · Cited by 527
Khan, A. H., Ghosh, S., Pradhan, B., Dalui, A., Shrestha, L. K., Acharya, S., & Ariga, K. (2017) · Bulletin of the Chemical Society of Japan · doi:10.1246/bcsj.20170043 · Cited by 432
Flexible graphene devices related to energy conversion and storage
Wang, X., & Shi, G. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03685a · Cited by 373
Lee, H. C., Liu, W.-W., Chai, S.-P., Mohamed, A. R., Aziz, A., Khe, C.-S., Hidayah, N. M. S., & Hashim, U. (2017) · RSC Advances · doi:10.1039/c7ra00392g · Cited by 357
Metadata
- Authors
- Li, W., Tan, C., Lowe, M. A., Abruña, H. D., & Ralph, D. C.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-02-18
- Volume
- 5
- Issue
- 3
- Pages
- 2264-2270
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2095114847
- Cited by
- 271
- References
- 1
- FWCI
- 12.55
- Type
- journal article
- Language
- en
- Open access
- closed
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