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High-Temperature Luminescence Quenching of Colloidal Quantum Dots
Open accessAbstract
Thermal quenching of quantum dot (QD) luminescence is important for application in luminescent devices. Systematic studies of the quenching behavior above 300 K are, however, lacking. Here, high-temperature (300-500 K) luminescence studies are reported for highly efficient CdSe core-shell quantum dots (QDs), aimed at obtaining insight into temperature quenching of QD emission. Through thermal cycling (yoyo) experiments for QDs in polymer matrices, reversible and irreversible luminescence quenching processes can be distinguished. For a variety of core-shell systems, reversible quenching is observed in a similar temperature range, between 100 and 180 °C. The irreversible quenching behavior varies between different systems. Mechanisms for thermal quenching are discussed.
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Skajaa, T., Zhao, Y., van den Heuvel, D. J., Gerritsen, H. C., Cormode, D. P., Koole, R., van Schooneveld, M. M., Post, J. A., Fisher, E. A., Fayad, Z. A., et al. (2010) · Nano Letters · doi:10.1021/nl1037903 · Cited by 76
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Luminescent probes and sensors for temperature
Wang, X.-D., Wolfbeis, O. S., & Meier, R. J. (2013) · Chemical Society Reviews · doi:10.1039/c3cs60102a · Cited by 1,647
Liang, Q., Ma, W., Shi, Y., Li, Z., & Yang, X. (2013) · Carbon · doi:10.1016/j.carbon.2013.04.055 · Cited by 658
Critical Red Components for Next-Generation White LEDs
Lin, C. C., Meijerink, A., & Liu, R.-S. (2016) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b02433 · Cited by 462
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Metadata
- Authors
- Zhao, Y., Riemersma, C., Pietra, F., Koole, R., de Mello Donegá, C., & Meijerink, A.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-09-24
- Volume
- 6
- Issue
- 10
- Pages
- 9058-9067
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1981830549
- Cited by
- 412
- References
- 1
- FWCI
- 7.53
- Type
- journal article
- Language
- en
- Open access
- green
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- Zhao, Y., Riemersma, C., Pietra, F., Koole, R., de Mello Donegá, C., & Meijerink, A. (2012). High-Temperature Luminescence Quenching of Colloidal Quantum Dots. ACS Nano. https://doi.org/10.1021/nn303217q
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