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Selenium@Mesoporous Carbon Composite with Superior Lithium and Sodium Storage Capacity
Abstract
Selenium-impregnated carbon composites were synthesized by infusing Se into mesoporous carbon at a temperature of 600 °C under vacuum. Ring-structured Se8 was produced and confined in the mesoporous carbon, which acts as an electronic conductive matrix. During the electrochemical process in low-cost LiPF6/EC/DEC electrolyte, low-order polyselenide intermediates formed and were stabilized by mesoporous carbon, which avoided the shuttle reaction of polyselenides. Exceptional electrochemical performance of Se/mesoporous carbon composites was demonstrated in both Li-ion and Na-ion batteries. In lithium-ion batteries, Se8/mesoporous carbon composite cathodes delivered a reversible capacity of 480 mAh g(-1) for 1000 charge/discharge cycles without any capacity loss, while in Na-ion batteries, it provided initial capacity of 485 mAh g(-1) and retained 340 mAh g(-1) after 380 cycles. The Se8/mesoporous carbon composites also showed excellent rate capability. As the current density increased from 0.1 to 5 C, the capacity retained about 46% in Li-ion batteries and 34% in Na-ion batteries.
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Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
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Lee, B., Paek, E., Mitlin, D., & Lee, S. W. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00642 · Cited by 940
Applications of Phosphorene and Black Phosphorus in Energy Conversion and Storage Devices
Pang, J., Bachmatiuk, A., Yin, Y., Trzebicka, B., Zhao, L., Fu, L., Mendes, R. G., Gemming, T., Liu, Z., & Rummeli, M. H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702093 · Cited by 518
Xu, J., Ma, J., Fan, Q., Guo, S., & Dou, S. (2017) · Advanced Materials · doi:10.1002/adma.201606454 · Cited by 319
Yang, J., Gao, H., Men, S., Shi, Z., Lin, Z., Kang, X., & Chen, S. (2018) · Advanced Science · doi:10.1002/advs.201800763 · Cited by 299
Wang, C., Wang, Z., Wu, D., Cai, W., Qin, Y., & Kong, Y. (2022) · Journal of Electroanalytical Chemistry · doi:10.1016/j.jelechem.2021.115976 · Cited by 33
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Metadata
- Authors
- Luo, C., Xu, Y., Zhu, Y., Liu, Y., Zheng, S., Liu, Y., Langrock, A., & Wang, C.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-08-19
- Volume
- 7
- Issue
- 9
- Pages
- 8003-8010
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2080891030
- Cited by
- 439
- References
- 1
- FWCI
- 23.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Luo, C., Xu, Y., Zhu, Y., Liu, Y., Zheng, S., Liu, Y., Langrock, A., & Wang, C. (2013). Selenium@Mesoporous Carbon Composite with Superior Lithium and Sodium Storage Capacity. ACS Nano. https://doi.org/10.1021/nn403108w
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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