The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
High-Performance Multifunctional Graphene Yarns: Toward Wearable All-Carbon Energy Storage Textiles
Open accessAbstract
The successful commercialization of smart wearable garments is hindered by the lack of fully integrated carbon-based energy storage devices into smart wearables. Since electrodes are the active components that determine the performance of energy storage systems, it is important to rationally design and engineer hierarchical architectures atboth the nano- and macroscale that can enjoy all of the necessary requirements for a perfect electrode. Here we demonstrate a large-scale flexible fabrication of highly porous high-performance multifunctional graphene oxide (GO) and rGO fibers and yarns by taking advantage of the intrinsic soft self-assembly behavior of ultralarge graphene oxide liquid crystalline dispersions. The produced yarns, which are the only practical form of these architectures for real-life device applications, were found to be mechanically robust (Young's modulus in excess of 29 GPa) and exhibited high native electrical conductivity (2508 ± 632 S m(-1)) and exceptionally high specific surface area (2605 m(2) g(-1) before reduction and 2210 m(2) g(-1) after reduction). Furthermore, the highly porous nature of these architectures enabled us to translate the superior electrochemical properties of individual graphene sheets into practical everyday use devices with complex geometrical architectures. The as-prepared final architectures exhibited an open network structure with a continuous ion transport network, resulting in unrivaled charge storage capacity (409 F g(-1) at 1 A g(-1)) and rate capability (56 F g(-1) at 100 A g(-1)) while maintaining their strong flexible nature.
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Cites
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Cited by
Carbon-Based Fibers for Advanced Electrochemical Energy Storage Devices
Chen, S., Qiu, L., & Cheng, H.-M. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00466 · Cited by 555
Materials Design and System Construction for Conventional and New‐Concept Supercapacitors
Wu, Z., Li, L., Yan, J., & Zhang, X. (2017) · Advanced Science · doi:10.1002/advs.201600382 · Cited by 470
Room-Temperature, Highly Durable Ti3C2Tx MXene/Graphene Hybrid Fibers for NH3 Gas Sensing
Lee, S. H., Eom, W., Shin, H., Ambade, R. B., Bang, J. H., Kim, H. W., & Han, T. H. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.9b21765 · Cited by 435
Ultrahigh‐Conductivity Polymer Hydrogels with Arbitrary Structures
Yao, B., Wang, H., Zhou, Q., Wu, M., Zhang, M., Li, C., & Shi, G. (2017) · Advanced Materials · doi:10.1002/adma.201700974 · Cited by 423
Flexible graphene devices related to energy conversion and storage
Wang, X., & Shi, G. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03685a · Cited by 373
Metadata
- Authors
- Aboutalebi, S. H., Jalili, R., Esrafilzadeh, D., Salari, M., Gholamvand, Z., Aminorroaya Yamini, S., Konstantinov, K., Shepherd, R. L., Chen, J., Moulton, S. E., Innis, P. C., Minett, A. I., Razal, J. M., & Wallace, G. G.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-02-17
- Volume
- 8
- Issue
- 3
- Pages
- 2456-2466
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2065084435
- Cited by
- 375
- References
- 37
- FWCI
- 15.37
- Type
- journal article
- Language
- en
- Open access
- green
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- Aboutalebi, S. H., Jalili, R., Esrafilzadeh, D., Salari, M., Gholamvand, Z., Aminorroaya Yamini, S., Konstantinov, K., Shepherd, R. L., Chen, J., Moulton, S. E., Innis, P. C., Minett, A. I., Razal, J. M., & Wallace, G. G. (2014). High-Performance Multifunctional Graphene Yarns: Toward Wearable All-Carbon Energy Storage Textiles. ACS Nano. https://doi.org/10.1021/nn406026z
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