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Cited by 375

The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.

High-Performance Multifunctional Graphene Yarns: Toward Wearable All-Carbon Energy Storage Textiles

Open access
Aboutalebi, Seyed Hamed, Jalili, Rouhollah, Esrafilzadeh, Dorna, Salari, Maryam, Gholamvand, Zahra, Aminorroaya Yamini, Sima, Konstantinov, Konstantin, Shepherd, Roderick L., Chen, Jun, Moulton, Simon E., Innis, Peter Charles, Minett, Andrew I., Razal, Joselito M., Wallace, Gordon G.·2014·ACS Nano
DOI 10.1021/nn406026z
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Abstract

The successful commercialization of smart wearable garments is hindered by the lack of fully integrated carbon-based energy storage devices into smart wearables. Since electrodes are the active components that determine the performance of energy storage systems, it is important to rationally design and engineer hierarchical architectures atboth the nano- and macroscale that can enjoy all of the necessary requirements for a perfect electrode. Here we demonstrate a large-scale flexible fabrication of highly porous high-performance multifunctional graphene oxide (GO) and rGO fibers and yarns by taking advantage of the intrinsic soft self-assembly behavior of ultralarge graphene oxide liquid crystalline dispersions. The produced yarns, which are the only practical form of these architectures for real-life device applications, were found to be mechanically robust (Young's modulus in excess of 29 GPa) and exhibited high native electrical conductivity (2508 ± 632 S m(-1)) and exceptionally high specific surface area (2605 m(2) g(-1) before reduction and 2210 m(2) g(-1) after reduction). Furthermore, the highly porous nature of these architectures enabled us to translate the superior electrochemical properties of individual graphene sheets into practical everyday use devices with complex geometrical architectures. The as-prepared final architectures exhibited an open network structure with a continuous ion transport network, resulting in unrivaled charge storage capacity (409 F g(-1) at 1 A g(-1)) and rate capability (56 F g(-1) at 100 A g(-1)) while maintaining their strong flexible nature.

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Metadata

Authors
Aboutalebi, S. H., Jalili, R., Esrafilzadeh, D., Salari, M., Gholamvand, Z., Aminorroaya Yamini, S., Konstantinov, K., Shepherd, R. L., Chen, J., Moulton, S. E., Innis, P. C., Minett, A. I., Razal, J. M., & Wallace, G. G.
Venue
ACS Nano
Publisher
American Chemical Society (ACS)
Published
2014-02-17
Volume
8
Issue
3
Pages
2456-2466
ISSN
  • 1936-0851 (ISSN-L)
  • 1936-086X
DOI
10.1021/nn406026z
OpenAlex
W2065084435
Cited by
375
References
37
FWCI
15.37
Type
journal article
Language
en
Open access
green

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