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Boron- and Nitrogen-Doped Graphene Quantum Dots/Graphene Hybrid Nanoplatelets as Efficient Electrocatalysts for Oxygen Reduction

Fei, Huilong, Ye, Ruquan, Ye, Gonglan, Gong, Yongji, Peng, Zhiwei, Fan, Xiujun, Samuel, Errol L. G., Ajayan, Pulickel M., Tour, James M.·2014·ACS Nano

Abstract

The scarcity and high cost of platinum-based electrocatalysts for the oxygen reduction reaction (ORR) has limited the commercial and scalable use of fuel cells. Heteroatom-doped nanocarbon materials have been demonstrated to be efficient alternative catalysts for ORR. Here, graphene quantum dots, synthesized from inexpensive and earth-abundant anthracite coal, were self-assembled on graphene by hydrothermal treatment to form hybrid nanoplatelets that were then codoped with nitrogen and boron by high-temperature annealing. This hybrid material combined the advantages of both components, such as abundant edges and doping sites, high electrical conductivity, and high surface area, which makes the resulting materials excellent oxygen reduction electrocatalysts with activity even higher than that of commercial Pt/C in alkaline media.

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Metadata

Authors
Fei, H., Ye, R., Ye, G., Gong, Y., Peng, Z., Fan, X., Samuel, E. L. G., Ajayan, P. M., & Tour, J. M.
Venue
ACS Nano
Published
2014-10-01
Volume
8
Issue
10
Pages
10837-10843
ISSN
  • 1936-0851 (ISSN-L)
  • 1936-086X
OpenAlex
W2065218823
Cited by
427
References
4
FWCI
15.28
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Boron- and Nitrogen-Doped Graphene Quantum Dots/Graphene Hybrid Nanoplatelets as Efficient Electrocatalysts for Oxygen Reduction. https://app.cochat.ai/papers/10.1021/nn504637y
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Fei, H., Ye, R., Ye, G., Gong, Y., Peng, Z., Fan, X., Samuel, E. L. G., Ajayan, P. M., & Tour, J. M. (2014). Boron- and Nitrogen-Doped Graphene Quantum Dots/Graphene Hybrid Nanoplatelets as Efficient Electrocatalysts for Oxygen Reduction. ACS Nano. https://doi.org/10.1021/nn504637y

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